Light Extraction Enhancement in Flexible Organic Light-Emitting Diodes by a Light-Scattering Layer of Dewetted Ag Nanoparticles at Low Temperatures

被引:36
作者
Choi, Junhee [1 ]
Kim, Seonju [1 ,3 ]
Park, Cheol Hwee [1 ]
Kwack, Jin Ho [1 ,3 ]
Park, Chan Hyuk [1 ]
Hwang, Ha [1 ]
Im, Hyeong-Seop [2 ]
Park, Young Wook [4 ]
Ju, Byeong-Kwon [1 ]
机构
[1] Korea Univ, Display & Nanosyst Lab, Dept Elect Engn, Seoul 02841, South Korea
[2] Korea Univ, Dept Mat Sci & Engn, Seoul 02841, South Korea
[3] Samsung Display Co, Samsung St 181, Asan 31454, Chungcheongnam, South Korea
[4] Sun Moon Univ, Sch Mech & ICT Convergence Engn, Asan 31460, Chungcheongnam, South Korea
基金
新加坡国家研究基金会;
关键词
organic light-emitting diodes (OLEDs); plasmonics; metal nanoparticles; light extraction; light scattering; SURFACE-PLASMON RESONANCE; SOLAR-CELLS; DELAYED FLUORESCENCE; EFFICIENT; DEVICES; OLEDS; INDEX; PEDOTPSS; FILMS; EMISSION;
D O I
10.1021/acsami.8b07026
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
We demonstrated light extraction improvement by applying a scattering layer of Ag nanoparticles physically synthesized through a low-temperature annealing process to flexible organic light-emitting diodes (OLEDs). In general, increasing the size of Ag nanoparticles is preferred to increase light scattering, but a high-temperature annealing process (similar to 400 degrees C) is required to produce them. However, flexible substrates generally cannot withstand high-temperature processes. In this study, we formed Ag nanoparticles at a low temperature of similar to 200 degrees C by inserting a poly(3,4-ethylenedioxythiophene) polystyrene sulfonate buffer layer, thus promoting Ag dewetting. As a result, the scattering layer of enlarged Ag nanoparticles formed at low temperatures increased the external quantum efficiency by 24% in a flexible OLED compared to a reference device.
引用
收藏
页码:32373 / 32379
页数:7
相关论文
共 52 条
[51]  
Zhang QS, 2014, NAT PHOTONICS, V8, P326, DOI [10.1038/NPHOTON.2014.12, 10.1038/nphoton.2014.12]
[52]   Hybrid Tamm plasmon-polariton/microcavity modes for white top-emitting organic light-emitting devices [J].
Zhang, Xu-Lin ;
Feng, Jing ;
Han, Xiao-Chi ;
Liu, Yue-Feng ;
Chen, Qi-Dai ;
Song, Jun-Feng ;
Sun, Hong-Bo .
OPTICA, 2015, 2 (06) :579-584