Flux calculation using CARIBIC DOAS aircraft measurements: SO2 emission of Norilsk

被引：23

作者：

Walter, D. ^{[1
,2
]}

Heue, K. -P. ^{[1
]}

Rauthe-Schoech, A. ^{[1
]}

Brenninkmeijer, C. A. M. ^{[1
]}

Lamsal, L. N. ^{[3
,4
]}

Krotkov, N. A. ^{[3
]}

Platt, U. ^{[2
]}

机构：

[1] Max Planck Inst Chem, DE-55128 Mainz, Germany

[2] Heidelberg Univ, Inst Environm Phys, Heidelberg, Germany

[3] NASA, Goddard Space Flight Ctr, Div Earth Sci, Atmospher Chem & Dynam Lab, Greenbelt, MD USA

[4] Univ Space Res Assoc, Columbia, MD USA

来源：

JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES | 2012年 / 117卷

关键词：

ABSORPTION CROSS-SECTIONS; GAS-PHASE REACTIONS; ATMOSPHERIC CHEMISTRY; PHOTOCHEMICAL DATA; SULFUR; OZONE; SPECTROSCOPY; MODEL; NO2; ERUPTION;

D O I：

10.1029/2011JD017335

中图分类号：

P4 [大气科学（气象学）];

学科分类号：

0706 ; 070601 ;

摘要：

Based on a case-study of the nickel smelter in Norilsk (Siberia), the retrieval of trace gas fluxes using airborne remote sensing is discussed. A DOAS system onboard an Airbus 340 detected large amounts of SO2 and NO2 near Norilsk during a regular passenger flight within the CARIBIC project. The remote sensing data were combined with ECMWF wind data to estimate the SO2 output of the Norilsk industrial complex to be around 1 Mt per year, which is in agreement with independent estimates. This value is compared to results using data from satellite remote sensing (GOME, OMI). The validity of the assumptions underlying our estimate is discussed, including the adaptation of this method to other gases and sources like the NO2 emissions of large industries or cities.

引用

页数：11

共 47 条

[1] Evaluated kinetic and photochemical data for atmospheric chemistry: Volume III - gas phase reactions of inorganic halogens [J].

Atkinson, R. ;

Baulch, D. L. ;

Cox, R. A. ;

Crowley, J. N. ;

Hampson, R. F. ;

Hynes, R. G. ;

Jenkin, M. E. ;

Rossi, M. J. ;

Troe, J. .

ATMOSPHERIC CHEMISTRY AND PHYSICS, 2007, 7 :981-1191

[2] Evaluated kinetic and photochemical data for atmospheric chemistry:: Volume I -: gas phase reactions of Ox, HOx, NOx and SOx species [J].

Atkinson, R ;

Baulch, DL ;

Cox, RA ;

Crowley, JN ;

Hampson, RF ;

Hynes, RG ;

Jenkin, ME ;

Rossi, MJ ;

Troe, J .

ATMOSPHERIC CHEMISTRY AND PHYSICS, 2004, 4 :1461-1738

[3]

Blacksmith Institutes, 2007, WORLDS WORST POLL PL

[4] Measurements of molecular absorption spectra with the SCIAMACHY pre-flight model: instrument characterization and reference data for atmospheric remote-sensing in the 230-2380 nm region [J].

Bogumil, K ;

Orphal, J ;

Homann, T ;

Voigt, S ;

Spietz, P ;

Fleischmann, OC ;

Vogel, A ;

Hartmann, M ;

Kromminga, H ;

Bovensmann, H ;

Frerick, J ;

Burrows, JP .

JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY, 2003, 157 (2-3) :167-184

[5]

Brasseur G., 1999, Atmospheric chemistry and global change

[6] Civil Aircraft for the regular investigation of the atmosphere based on an instrumented container: The new CARIBIC system [J].

Brenninkmeijer, C. A. M. ;

Crutzen, P. ;

Boumard, F. ;

Dauer, T. ;

Dix, B. ;

Ebinghaus, R. ;

Filippi, D. ;

Fischer, H. ;

Franke, H. ;

Friess, U. ;

Heintzenberg, J. ;

Helleis, F. ;

Hermann, M. ;

Kock, H. H. ;

Koeppel, C. ;

Lelieveld, J. ;

Leuenberger, M. ;

Martinsson, B. G. ;

Miemczyk, S. ;

Moret, H. P. ;

Nguyen, H. N. ;

Nyfeler, P. ;

Oram, D. ;

O'Sullivan, D. ;

Penkett, S. ;

Platt, U. ;

Pupek, M. ;

Ramonet, M. ;

Randa, B. ;

Reichelt, M. ;

Rhee, T. S. ;

Rohwer, J. ;

Rosenfeld, K. ;

Scharffe, D. ;

Schlager, H. ;

Schumann, U. ;

Slemr, F. ;

Sprung, D. ;

Stock, P. ;

Thaler, R. ;

Valentino, F. ;

van Velthoven, P. ;

Waibel, A. ;

Wandel, A. ;

Waschitschek, K. ;

Wiedensohler, A. ;

Xueref-Remy, I. ;

Zahn, A. ;

Zech, U. ;

Ziereis, H. .

ATMOSPHERIC CHEMISTRY AND PHYSICS, 2007, 7 (18) :4953-4976

[7]

Burrows JP, 1999, J ATMOS SCI, V56, P151, DOI 10.1175/1520-0469(1999)056<0151:TGOMEG>2.0.CO

[8]

[9]

Bussemer M., 1993, Der Ring-Effekt: Ursachen und Einfluss auf die spektroskopische Messung stratosphaerischer Spurenstoffe

[10] Opportunistic validation of sulfur dioxide in the Sarychev Peak volcanic eruption cloud [J].

Carn, S. A. ;

Lopez, T. M. .

ATMOSPHERIC MEASUREMENT TECHNIQUES, 2011, 4 (09) :1705-1712

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