Low-bandgap thieno[3,4-c]pyrrole-4,6-dione-polymers for high-performance solar cells with significantly enhanced photocurrents

被引：34
作者：
Zhang, Cheng [1 ]
Li, Hui [1 ]
Wang, Jizheng [1 ]
Zhang, Yongfang [1 ]
Qiao, Yan [3 ]
Huang, Dazhen [1 ]
Di, Chong-an [1 ]
Zhan, Xiaowei [2 ]
Zhu, Xiaozhang [1 ]
Zhu, Daoben [1 ]
机构：
[1] Chinese Acad Sci, Inst Chem, CAS Key Lab Organ Solids, Beijing Natl Lab Mol Sci, Beijing 100080, Peoples R China
[2] Peking Univ, Coll Engn, Dept Mat Sci & Engn, Beijing 100871, Peoples R China
[3] Chinese Acad Sci, Inst Coal Chem, State Key Lab Coal Convers, Taiyuan 030001, Shanxi, Peoples R China
来源：
JOURNAL OF MATERIALS CHEMISTRY A | 2015年 / 3卷 / 21期
基金：
中国国家自然科学基金;
关键词：
CONJUGATED POLYMERS; PHOTOVOLTAIC PERFORMANCE; ALTERNATING COPOLYMERS; DEVICE PERFORMANCE; MOLECULAR DESIGN; RATIONAL DESIGN; BUILDING-BLOCK; TANDEM POLYMER; SUBSTITUTION; EFFICIENCY;
D O I：
10.1039/c5ta02376a
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Low-bandgap thieno[3,4-c]pyrrole-4,6-dione-polymers with proximal and distal configurations were synthesized for polymer solar cells. Photovoltaic performance depends on the orientation of the fused thiophene subunits, which is related to the different semiconducting properties and phase separation. Without special device treatments, P3 showed power conversion efficiencies of up to 7.50% with the highest short-circuit current (J(sc) = 18.2 mA cm(-2)) so far reported for TPD polymers.
引用
收藏
页码：11194 / 11198
页数：5
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  • [1] Highly efficient organic tandem solar cells: a follow up review
    Ameri, Tayebeh
    Li, Ning
    Brabec, Christoph J.
    [J]. ENERGY & ENVIRONMENTAL SCIENCE, 2013, 6 (08) : 2390 - 2413
  • [2] Molecular Design and Ordering Effects in π-Functional Materials for Transistor and Solar Cell Applications
    Beaujuge, Pierre M.
    Frechet, Jean M. J.
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2011, 133 (50) : 20009 - 20029
  • [3] Synthesis and Characterization of 5-Octylthieno[3,4-c]pyrrole-4,6-dione Derivatives As New Monomers for Conjugated Copolymers
    Berrouard, Philippe
    Grenier, Francois
    Pouliot, Jean-Remi
    Gagnon, Eric
    Tessier, Christian
    Leclerc, Mario
    [J]. ORGANIC LETTERS, 2011, 13 (01) : 38 - 41
  • [4] Poly(diketopyrrolopyrrole-terthiophene) for Ambipolar Logic and Photovoltaics
    Bijleveld, Johan C.
    Zoombelt, Arjan P.
    Mathijssen, Simon G. J.
    Wienk, Martijn M.
    Turbiez, Mathieu
    de Leeuw, Dago M.
    Janssen, Rene A. J.
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2009, 131 (46) : 16616 - +
  • [5] Polymer-Fullerene Bulk-Heterojunction Solar Cells
    Brabec, Christoph J.
    Gowrisanker, Srinivas
    Halls, Jonathan J. M.
    Laird, Darin
    Jia, Shijun
    Williams, Shawn P.
    [J]. ADVANCED MATERIALS, 2010, 22 (34) : 3839 - 3856
  • [6] Linear Side Chains in Benzo[1,2-b:4,5-b′]dithiophene-Thieno[3,4-c]pyrrole-4,6-dione Polymers Direct Self-Assembly and Solar Cell Performance
    Cabanetos, Clement
    El Labban, Abdulrahman
    Bartelt, Jonathan A.
    Douglas, Jessica D.
    Mateker, William R.
    Frechet, Jean M. J.
    McGehee, Michael D.
    Beaujuge, Pierre M.
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2013, 135 (12) : 4656 - 4659
  • [7] Bulk Heterojunction Solar Cells Using Thieno[3,4-c]pyrrole-4,6-dione and Dithieno[3,2-b:2′,3′-d]silole Copolymer with a Power Conversion Efficiency of 7.3%
    Chu, Ta-Ya
    Lu, Jianping
    Beaupre, Serge
    Zhang, Yanguang
    Pouliot, Jean-Remi
    Wakim, Salem
    Zhou, Jiayun
    Leclerc, Mario
    Li, Zhao
    Ding, Jianfu
    Tao, Ye
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2011, 133 (12) : 4250 - 4253
  • [8] 25th Anniversary Article: A Decade of Organic/Polymeric Photovoltaic Research
    Dou, Letian
    You, Jingbi
    Hong, Ziruo
    Xu, Zheng
    Li, Gang
    Street, Robert A.
    Yang, Yang
    [J]. ADVANCED MATERIALS, 2013, 25 (46) : 6642 - 6671
  • [9] Synthesis of 5H-Dithieno[3,2-b:2′,3′-d]pyran as an Electron-Rich Building Block for Donor-Acceptor Type Low-Bandgap Polymers
    Dou, Letian
    Chen, Chun-Chao
    Yoshimura, Ken
    Ohya, Kenichiro
    Chang, Wei-Hsuan
    Gao, Jing
    Liu, Yongsheng
    Richard, Eric
    Yang, Yang
    [J]. MACROMOLECULES, 2013, 46 (09) : 3384 - 3390
  • [10] A Selenium-Substituted Low-Bandgap Polymer with Versatile Photovoltaic Applications
    Dou, Letian
    Chang, Wei-Hsuan
    Gao, Jing
    Chen, Chun-Chao
    You, Jingbi
    Yang, Yang
    [J]. ADVANCED MATERIALS, 2013, 25 (06) : 825 - 831
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