Graphene oxide modified waste newspaper for removal of heavy metal ions and its application in industrial wastewater

被引:41
作者
Chen, Hang [1 ]
Meng, Yi [1 ]
Jia, Shiyao [1 ]
Hua, Wenqiang [1 ]
Cheng, Yi [1 ]
Lu, Jie [1 ]
Wang, Haisong [1 ]
机构
[1] Dalian Polytech Univ, Sch Light Ind & Chem Engn, Dalian 116034, Peoples R China
基金
国家重点研发计划;
关键词
Graphene oxide; Assembled paper; Absorption capacity; Bleaching effluent; AQUEOUS-SOLUTION; ACTIVATED CARBON; METHYLENE-BLUE; EFFICIENT REMOVAL; LOW-COST; PB(II) IONS; ADSORPTION; ADSORBENT; NANOSHEETS; GRAPHITE;
D O I
10.1016/j.matchemphys.2020.122692
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Waste newspapers as absorbents to remove contaminant are limit to the extracting fibers from the newspaper at present, which lead to a complicated preparation and a difficult separation at the end of adsorption. In this study, we reported a simple, effective and renewable adsorption material assembled with waste newspaper and graphene oxide (GO). The adsorption and durability of the GO/paper have been evaluated using heavy metal ions solution and industrial effluent from the bleaching plant of paper industry, and the adsorption isotherm and kinetics are also valuated. The results indicate that the maximum adsorption capacities of GO/paper are 75.41 mg/g, 29.04 mg/g and 31.35 mg/g for Pb2+, Ni2+ and Cd2+, respectively, and the regeneration efficiency of the adsorbent to each ion is reduced by less than 10% within three testing cycles. Moreover, the GO/paper has a superior performance of removing the residual lignin and Chemical Oxygen Demand of the bleaching effluent, the adsorption of which are 64.4 mg/g and 225.7 mg/g, respectively. All these results highlight that the GO/paper as an environment-friendly, renewable and low-cost material possess an excellent adsoThe issue of water pollution is a stubborn hidden danger and damage to the environment in many industries [1]. The accumulation of toxicrption capacity for both heavy metal ions and industrial wastewater.
引用
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页数:10
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共 71 条
[1]   Efficient removal of toxic bromothymol blue and methylene blue from wastewater by polyvinyl alcohol [J].
Agarwal, Shilpi ;
Sadegh, Hamidreza ;
Monajjemi, Majid ;
Hamdy, Abdel Salam ;
Ali, Gomaa A. M. ;
Memar, Amir O. H. ;
Shahryari-ghoshekandi, Ramin ;
Tyagi, Inderjeet ;
Gupta, Vinod Kumar .
JOURNAL OF MOLECULAR LIQUIDS, 2016, 218 :191-197
[2]   New magnetic silica-based hybrid organic-inorganic nanocomposite for the removal of lead(II) and nickel(II) ions from aqueous solutions [J].
Ahmad, Naqhiyah ;
Sereshti, Hassan ;
Mousazadeh, Milad ;
Nodeh, Hamid Rashidi ;
Kamboh, Muhammad Afzal ;
Mohamad, Sharifah .
MATERIALS CHEMISTRY AND PHYSICS, 2019, 226 :73-81
[3]   Removal of heavy metal ions by nanofiltration [J].
Al-Rashdi, B. A. M. ;
Johnson, D. J. ;
Hilal, N. .
DESALINATION, 2013, 315 :2-17
[4]   Activated lignin-chitosan extruded blends for efficient adsorption of methylene blue [J].
Albadarin, Ahmad B. ;
Collins, Maurice N. ;
Naushad, Mu ;
Shirazian, Saeed ;
Walker, Gavin ;
Mangwandi, C. .
CHEMICAL ENGINEERING JOURNAL, 2017, 307 :264-272
[5]   Potential of using green adsorbent of heavy metal removal from aqueous solutions: Adsorption kinetics, isotherm, thermodynamic, mechanism and economic analysis [J].
Ali, Rehab M. ;
Hamad, Hesham A. ;
Hussein, Mohamed M. ;
Malash, Gihan F. .
ECOLOGICAL ENGINEERING, 2016, 91 :317-332
[6]   Preparation, characterization and evaluation of bio-based magnetic activated carbon for effective adsorption of malachite green from aqueous solution [J].
Altintig, Esra ;
Onaran, Muge ;
Sari, Ahmet ;
Altundag, Huseyin ;
Tuzen, Mustafa .
MATERIALS CHEMISTRY AND PHYSICS, 2018, 220 :313-321
[7]   Removal of congo red azo dye from aqueous solution by ZnO nanoparticles loaded on multiwall carbon nanotubes [J].
Arabi, Seyed Masoud Seyed ;
Lalehloo, Rahman Shakibaei ;
Olyai, Mohamad Reza Talei Bavil ;
Ali, Gomaa A. M. ;
Sadegh, Hamidreza .
PHYSICA E-LOW-DIMENSIONAL SYSTEMS & NANOSTRUCTURES, 2019, 106 :150-155
[8]   Synthesis of a new nanocomposite based-on graphene-oxide for selective removal of Pb2+ ions from aqueous solutions [J].
Avval, Mahsa Ensafi ;
Moghadam, Peyman Najafi ;
Baradarani, Mohammad Mehdi .
POLYMER COMPOSITES, 2019, 40 (02) :730-737
[9]   Efficient Removal of Heavy Metals from Polluted Water with High Selectivity for Mercury(II) by 2-lmino-4-thiobiuret-Partially Reduced Graphene Oxide (IT-PRGO) [J].
Awad, Fathi S. ;
AbouZeid, Khaled M. ;
Abou El-Maaty, Weam M. ;
El-Wakil, Ahmad M. ;
El Shall, M. Samy .
ACS APPLIED MATERIALS & INTERFACES, 2017, 9 (39) :34230-34242
[10]   Removal of copper (II) from aqueous solution by adsorption onto low-cost adsorbents [J].
Aydin, Haluk ;
Buluta, Yasemin ;
Yerlikaya, Cigdem .
JOURNAL OF ENVIRONMENTAL MANAGEMENT, 2008, 87 (01) :37-45