Recent progress in carbon-based materials boosting electrochemical water splitting

As environmental crises such as global warming become more and more serious due to the large amount of carbon dioxide emitted by the burning of fossil fuels, much attention has been paid to carbon neutrality. Hydrogen, with zero carbon content, is a clean and renewable energy carrier having a large energy density. It is considered as one of the most desirable alternatives to fossil fuels. Electrochemical water splitting, unlike the steam reforming process accelerating fossil fuels depletion and CO2 emissions, can produce H-2 powered by renewable energy such as solar or wind. As a promising way to promote carbon neutralization, hydrogen production by electrolysis of water is meaningful both in terms of scientific research and practical application. In order to drive electrochemical water splitting with low power consumption, efficient, durable and affordable electrocatalysts with low overpotentials are in urgent need. Therefore, this mini-review briefly introduces the current development status and mainstream obstacles of carbon-based materials used in electrochemical water splitting. (C) 2022 Published by Elsevier B.V. on behalf of Chinese Chemical Society and Institute of Materia Medica, Chinese Academy of Medical Sciences.