Flexible Low-Temperature Ammonia Gas Sensor Based on Reduced Graphene Oxide and Molybdenum Disulfide

被引:19
作者
Ren, Zhe [1 ]
Shi, Yunbo [1 ]
Song, Tianming [1 ]
Wang, Tian [1 ]
Tang, Bolun [1 ]
Niu, Haodong [1 ]
Yu, Xiaoyu [2 ]
机构
[1] Harbin Univ Sci & Technol, Higher Educ Key Lab Measuring & Control Technol &, Harbin 150080, Peoples R China
[2] Sun Yat Sen Univ, Sch Atmospher Sci, Guangzhou 519000, Peoples R China
基金
美国国家科学基金会;
关键词
flexible electronics; micro-electro-mechanical system; reduced graphene oxide; NH3 gas sensor; molybdenum disulfide; HIGHLY TRANSPARENT; LAYER MOS2; PERFORMANCE; STRAIN;
D O I
10.3390/chemosensors9120345
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
Owing to harsh working environments and complex industrial requirements, traditional gas sensors are prone to deformation damage, possess a limited detection range, require a high working temperature, and display low reliability, thereby necessitating the development of flexible and low-temperature gas sensors. In this study, we developed a low-temperature polyimide (PI)-based flexible gas sensor comprising a reduced graphene oxide (rGO)/MoS2 composite. The micro-electro-mechanical system technology was used to fabricate Au electrodes on a flexible PI sheet to form a "sandwiched" sensor structure. The rGO/MoS2 composites were synthesized via a one-step hydrothermal method. The gas-sensing response was the highest for the composite comprising 10% rGO. The structure of this material was characterized, and a PI-based flexible gas sensor comprising rGO/MoS2 was fabricated. The optimal working temperature of the sensor was 141 degrees C, and its response-recovery time was significantly short upon exposure to 50-1500 ppm NH3. Thus, this sensor exhibited high selectivity and a wide NH3 detection range. Furthermore, it possessed the advantages of low power consumption, a short response-recovery time, a low working temperature, flexibility, and variability. Our findings provide a new framework for the development of pollutant sensors that can be utilized in an industrial environment.
引用
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页数:16
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