Ultrafast temporal evolution of interatomic Coulombic decay in NeKr dimers

被引：3

作者：

Trinter, F. ^{[1
,2
]}

Miteva, T. ^{[3
]}

Weller, M. ^{[1
,4
]}

Hartung, A. ^{[1
]}

Richter, M. ^{[1
]}

Williams, J. B. ^{[5
]}

Gatton, A. ^{[4
,6
]}

Gaire, B. ^{[4
]}

Sartor, J. ^{[6
]}

Berry, B. ^{[7
]}

Ben-Itzhak, I. ^{[7
]}

Sisourat, N. ^{[3
]}

Stumpf, V ^{[8
]}

Gokhberg, K. ^{[8
]}

Doerner, R. ^{[1
]}

Jahnke, T. ^{[9
]}

Weber, T. ^{[4
]}

机构：

[1] Goethe Univ, Inst Kernphys, D-60438 Frankfurt, Germany

[2] Max Planck Gesell, Mol Phys, Fritz Haber Inst, D-14195 Berlin, Germany

[3] Sorbonne Univ, Lab Chim Phys Matiere & Rayonnement, CNRS, UMR 7614, F-75005 Paris, France

[4] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA

[5] Univ Nevada, Dept Phys, Reno, NV 89557 USA

[6] Auburn Univ, Dept Phys, Auburn, AL 36849 USA

[7] Kansas State Univ, Dept Phys, JR Macdonald Lab, Manhattan, KS 66506 USA

[8] Heidelberg Univ, Phys Chem Inst, Theoret Chem, D-69120 Heidelberg, Germany

[9] European XFEL GmbH, D-22869 Schenefeld, Germany

来源：

CHEMICAL SCIENCE | 2022年 / 13卷 / 06期

基金：

欧洲研究理事会;

关键词：

LOW-ENERGY ELECTRONS; DIATOMIC-MOLECULES; MOMENTUM SPECTROSCOPY; NOBLE-GASES; RECOIL-ION; PARTICLE; REPRESENTATION; FRAGMENTATION; DYNAMICS; STATE;

D O I：

10.1039/d1sc04630f

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

We investigate interatomic Coulombic decay in NeKr dimers after neon inner-valence photoionization [Ne+(2s(-1))] using a synchrotron light source. We measure with high energy resolution the two singly charged ions of the Coulomb-exploding dimer dication and the photoelectron in coincidence. By carefully tracing the post-collision interaction between the photoelectron and the emitted ICD electron we are able to probe the temporal evolution of the state as it decays. Although the ionizing light pulses are 80 picoseconds long, we determine the lifetime of the intermediate dimer cation state and visualize the contraction of the nuclear structure on the femtosecond time scale.

引用

页码：1789 / 1800

页数：12

共 50 条

[1] Interatomic Coulombic decay in mixed NeKr clusters
Arion, Tiberiu
Mucke, Melanie
Foerstel, Marko
Bradshaw, Alex M.
Hergenhahn, Uwe
JOURNAL OF CHEMICAL PHYSICS, 2011, 134 (07)
[2] Evolution of Interatomic Coulombic Decay in the Time Domain
Trinter, F.
Williams, J. B.
Weller, M.
Waitz, M.
Pitzer, M.
Voigtsberger, J.
Schober, C.
Kastirke, G.
Mueller, C.
Goihl, C.
Burzynski, P.
Wiegandt, F.
Bauer, T.
Wallauer, R.
Sann, H.
Kalinin, A.
Schmidt, L. Ph. H.
Schoeffler, M.
Sisourat, N.
Jahnke, T.
PHYSICAL REVIEW LETTERS, 2013, 111 (09)
[3] Experimental investigation of the interatomic Coulombic decay in NeAr dimers
O'Keeffe, P.
Ciavardini, A.
Ripani, E.
Bolognesi, P.
Coreno, M.
Avaldi, L.
Devetta, M.
Di Fraia, M.
Callegari, C.
Prince, K. C.
Richter, R.
PHYSICAL REVIEW A, 2014, 90 (04):
[4] Interatomic-Coulombic-decay-induced recapture of photoelectrons in helium dimers
Burzynski, P.
Trinter, F.
Williams, J. B.
Weller, M.
Waitz, M.
Pitzer, M.
Voigtsberger, J.
Schober, C.
Kastirke, G.
Mueller, C.
Goihl, C.
Wiegandt, F.
Wallauer, R.
Kalinin, A.
Schmidt, L. Ph H.
Schoeffler, M.
Schiwietz, G.
Sisourat, N.
Jahnke, T.
Doerner, R.
PHYSICAL REVIEW A, 2014, 90 (02):
[5] Interference effects in the photoelectron spectrum of the NeKr dimer and vibrationally selected interatomic Coulombic decay
Fedyk, Jacqueline
Gokhberg, Kirill
Miteva, Tsveta
Cederbaum, Lorenz S.
Kuleff, Alexander I.
PHYSICAL REVIEW A, 2023, 107 (02)
[6] Interatomic Coulombic decay of fixed-in-space neon dimers
Semenov, S. K.
Kreidi, K.
Jahnke, T.
Weber, Th.
Havermeier, T.
Grisenti, R. E.
Liu, X.
Morisita, Y.
Schmidt, L. Ph H.
Schoeffler, M. S.
Odenweller, M.
Neumann, N.
Foucar, L.
Titze, J.
Ulrich, B.
Sturm, F.
Kim, H. K.
Ueda, K.
Czasch, A.
Jagutzki, O.
Cherepkov, N. A.
Doerner, R.
PHYSICAL REVIEW A, 2012, 85 (04):
[7] Interatomic Coulombic Decay of HeNe dimers after ionization and excitation of He and Ne
Sann, H.
Havermeier, T.
Kim, H. -K.
Sturm, F.
Trinter, F.
Waitz, M.
Zeller, S.
Ulrich, B.
Meckel, M.
Voss, S.
Bauer, T.
Schneider, D.
Schmidt-Boecking, H.
Wallauer, R.
Schoeffler, M.
Williams, J. B.
Doerner, R.
Jahnke, T.
CHEMICAL PHYSICS, 2017, 482 : 221 - 225
[8] Ion-impact-induced interatomic Coulombic decay in neon and argon dimers
Kim, H. -K.
Gassert, H.
Schoeffler, M. S.
Titze, J. N.
Waitz, M.
Voigtsberger, J.
Trinter, F.
Becht, J.
Kalinin, A.
Neumann, N.
Zhou, C.
Schmidt, L. Ph. H.
Jagutzki, O.
Czasch, A.
Merabet, H.
Schmidt-Boecking, H.
Jahnke, T.
Cassimi, A.
Doerner, R.
PHYSICAL REVIEW A, 2013, 88 (04)
[9] Interatomic Coulombic decay in small helium clusters
Kazandjian, Sevan
Kircher, Max
Kastirke, Gregor
Williams, Joshua B.
Schoeffler, Markus
Kunitski, Maksim
Doerner, Reinhard
Miteva, Tsveta
Engin, Selma
Trinter, Florian
Jahnke, Till
Sisourat, Nicolas
PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2023, 25 (37) : 25711 - 25719
[10] Giant Interatomic Coulombic Decay
Sisourat, Nicolas
Kryzhevoi, Nikolai V.
Kolorenc, Premysl
Scheit, Simona
Cederbaum, Lorenz S.
XXVII INTERNATIONAL CONFERENCE ON PHOTONIC, ELECTRONIC AND ATOMIC COLLISIONS (ICPEAC 2011), PTS 1-15, 2012, 388

← 1 2 3 4 5 →