Enhanced flexoelectricity through residual ferroelectricity in barium strontium titanate

被引:60
作者
Garten, Lauren M. [1 ]
Trolier-McKinstry, Susan
机构
[1] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA
关键词
PHASE-TRANSITIONS; THIN-FILMS; POLARIZATION; SRTIO3; RAMAN;
D O I
10.1063/1.4913858
中图分类号
O59 [应用物理学];
学科分类号
摘要
Residual ferroelectricity is observed in barium strontium titanate ceramics over 30 degrees C above the global phase transition temperature, in the same temperature range in which anomalously large flexoelectric coefficients are reported. The application of a strain gradient leads to strain gradient-induced poling or flexoelectric poling. This was observed by the development of a remanent polarization in flexoelectric measurements, an induced d(33) piezoelectric response even after the strain gradient was removed, and the production of an internal bias of 9 kV m(-1). It is concluded that residual ferroelectric response considerably enhances the observed flexoelectric response. (C) 2015 AIP Publishing LLC.
引用
收藏
页数:5
相关论文
共 47 条
[1]   Formation and relaxation mechanisms of the self-polarization in thin ferroelectric films [J].
Afanas'ev, V. P. ;
Pronin, I. P. ;
Kholkin, A. L. .
PHYSICS OF THE SOLID STATE, 2006, 48 (06) :1214-1218
[2]   Polar precursor ordering in BaTiO3 detected by resonant piezoelectric spectroscopy [J].
Aktas, Oktay ;
Carpenter, Michael A. ;
Salje, Ekhard K. H. .
APPLIED PHYSICS LETTERS, 2013, 103 (14)
[3]  
Bassiri Gharb N., 2005, THESIS U PARK PENNSY
[4]   Domain wall contributions to the properties of piezoelectric thin films [J].
Bassiri-Gharb, Nazanin ;
Fujii, Ichiro ;
Hong, Eunki ;
Trolier-McKinstry, Susan ;
Taylor, David V. ;
Damjanovic, Dragan .
JOURNAL OF ELECTROCERAMICS, 2007, 19 (01) :49-65
[5]  
Biancoli A, 2015, NAT MATER, V14, P224, DOI [10.1038/NMAT4139, 10.1038/nmat4139]
[6]   Precursor effects, broken local symmetry, and coexistence of order-disorder and displacive dynamics in perovskite ferroelectrics [J].
Bussmann-Holder, A. ;
Beige, H. ;
Voelkel, G. .
PHYSICAL REVIEW B, 2009, 79 (18)
[7]  
Catalan G, 2011, NAT MATER, V10, P963, DOI [10.1038/nmat3141, 10.1038/NMAT3141]
[8]   Upward ferroelectric self-polarization induced by compressive epitaxial strain in (001) BaTiO3 films [J].
Chen, Jiangpeng ;
Luo, Ying ;
Ou, Xin ;
Yuan, Guoliang ;
Wang, Yiping ;
Yang, Ying ;
Yin, Jiang ;
Liu, Zhiguo .
JOURNAL OF APPLIED PHYSICS, 2013, 113 (20)
[9]   Flexoelectric effects: Charge separation in insulating solids subjected to elastic strain gradients [J].
Cross, LE .
JOURNAL OF MATERIALS SCIENCE, 2006, 41 (01) :53-63
[10]   Micro-Raman study of Ba1-xSrxTiO3 ceramics [J].
Dobal, PS ;
Dixit, A ;
Katiyar, RS ;
Garcia, D ;
Guo, R ;
Bhalla, AS .
JOURNAL OF RAMAN SPECTROSCOPY, 2001, 32 (02) :147-149