SALSA2.0: The sectional aerosol module of the aerosol-chemistry-climate model ECHAM6.3.0-HAM2.3-MOZ1.0

被引：58

作者：

Kokkola, Harri ^{[1
]}

Kuhn, Thomas ^{[1
,2
]}

Laakso, Anton ^{[1
,3
]}

Bergman, Tommi ^{[4
]}

Lehtinen, Kari E. J. ^{[1
,2
]}

Mielonen, Tero ^{[1
]}

Arola, Antti ^{[1
]}

Stadtler, Scarlet ^{[5
]}

Korhonen, Hannele ^{[6
]}

Ferrachat, Sylvaine ^{[7
]}

Lohmann, Ulrike ^{[7
]}

Neubauer, David ^{[7
]}

Tegen, Ina ^{[8
]}

Siegenthaler-Le Drian, Colombe ^{[9
]}

Schultz, Martin G. ^{[5
,10
]}

Bey, Isabelle ^{[9
,11
]}

Stier, Philip ^{[12
]}

Daskalakis, Nikos ^{[13
]}

Heald, Colette L. ^{[14
]}

Romakkaniemi, Sami ^{[1
]}

机构：

[1] Finnish Meteorol Inst, Atmospher Res Ctr Eastern Finland, POB 1627, Kuopio 70211, Finland

[2] Univ Eastern Finland, Aerosol Phys Res Grp, POB 1627, Kuopio 70211, Finland

[3] Univ Minnesota, Dept Soil Water & Climate, St Paul, MN 55108 USA

[4] Royal Netherlands Meteorol Inst, Weather & Climate Models, POB 201, NL-3730 AE De Bilt, Netherlands

[5] Forschungszentrum Julich, Inst Energie & Klimaforsch, IEK 8, Julich, Germany

[6] Finnish Meteorol Inst, Climate Res, Helsinki 00100, Finland

[7] Swiss Fed Inst Technol, Inst Atmospher & Climate Sci, CH-8092 Zurich, Switzerland

[8] Leibniz Inst Tropospher Res TROPOS, Modeling Atmospher Proc, Leipzig, Germany

[9] Swiss Fed Inst Technol, Ctr Climate Syst Modeling C2SM, Zurich, Switzerland

[10] Forschungszentrum Julich, JSC, Julich, Germany

[11] Ctr Meteorol Geneve, Off Fed Meteorol & Climatol MeteoSuisse, Av Paix 7bis, CH-1211 Geneva 2, Switzerland

[12] Univ Oxford, Dept Phys, Parks Rd, Oxford OX1 3PU, England

[13] Univ Bremen, Inst Environm Phys IUP, Lab Modeling & Observat Earth Syst LAMOS, Bremen, Germany

[14] MIT, Dept Earth Atmospher & Planetary Sci, Dept Civil & Environm Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA

来源：

GEOSCIENTIFIC MODEL DEVELOPMENT | 2018年 / 11卷 / 09期

基金：

芬兰科学院; 欧洲研究理事会; 美国国家科学基金会;

关键词：

SECONDARY ORGANIC AEROSOL; BIOMASS BURNING EMISSIONS; STRATOSPHERIC AEROSOL; CHEMICAL-COMPOSITION; PINATUBO ERUPTION; SIZE DISTRIBUTION; SULFURIC-ACID; OPTICAL DEPTH; MICROPHYSICS; SIMULATION;

D O I：

10.5194/gmd-11-3833-2018

中图分类号：

P [天文学、地球科学];

学科分类号：

07 ;

摘要：

In this paper, we present the implementation and evaluation of the aerosol microphysics module SALSA2.0 in the framework of the aerosol-chemistry-climate model ECHAM-HAMMOZ. It is an alternative microphysics module to the default modal microphysics scheme M7 in ECHAM-HAMMOZ. The SALSA2.0 implementation within ECHAM-HAMMOZ is evaluated against observations of aerosol optical properties, aerosol mass, and size distributions, comparing also to the skill of the M7 implementation. The largest differences between the implementation of SALSA2.0 and M7 are in the methods used for calculating microphysical processes, i.e., nucleation, condensation, coagulation, and hydration. These differences in the microphysics are reflected in the results so that the largest differences between SALSA2.0 and M7 are evident over regions where the aerosol size distribution is heavily modified by the microphysical processing of aerosol particles. Such regions are, for example, highly polluted regions and regions strongly affected by biomass burning. In addition, in a simulation of the 1991 Mt. Pinatubo eruption in which a stratospheric sulfate plume was formed, the global burden and the effective radii of the stratospheric aerosol are very different in SALSA2.0 and M7. While SALSA2.0 was able to reproduce the observed time evolution of the global burden of sulfate and the effective radii of stratospheric aerosol, M7 strongly overestimates the removal of coarse stratospheric particles and thus underestimates the effective radius of stratospheric aerosol. As the mode widths of M7 have been optimized for the troposphere and were not designed to represent stratospheric aerosol, the ability of M7 to simulate the volcano plume was improved by modifying the mode widths, decreasing the standard deviations of the accumulation and coarse modes from 1.59 and 2.0, respectively, to 1.2 similar to what was observed after the Mt. Pinatubo eruption. Overall, SALSA2.0 shows promise in improving the aerosol description of ECHAM-HAMMOZ and can be further improved by implementing methods for aerosol processes that are more suitable for the sectional method, e.g., size-dependent emissions for aerosol species and size-resolved wet deposition.

引用

页码：3833 / 3863

页数：31

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