Origin and radiative forcing of black carbon transported to the Himalayas and Tibetan Plateau

被引:170
作者
Kopacz, M. [1 ]
Mauzerall, D. L. [1 ,2 ]
Wang, J. [3 ]
Leibensperger, E. M. [4 ]
Henze, D. K. [5 ]
Singh, K. [6 ]
机构
[1] Princeton Univ, Woodrow Wilson Sch Publ & Int Affairs, Princeton, NJ 08544 USA
[2] Princeton Univ, Dept Civil & Environm Engn, Princeton, NJ 08544 USA
[3] Univ Nebraska, Dept Earth & Atmospher Sci, Lincoln, NE USA
[4] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA
[5] Univ Colorado, Dept Mech Engn, Boulder, CO 80309 USA
[6] Virginia Polytech Inst & State Univ, Dept Comp Sci, Blacksburg, VA USA
关键词
INTERANNUAL VARIABILITY; OZONE POLLUTION; AIR-QUALITY; SNOW; SATELLITE; CLIMATE; AIRCRAFT; ADJOINT; MODEL; EMISSIONS;
D O I
10.5194/acp-11-2837-2011
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The remote and high elevation regions of central Asia are influenced by black carbon (BC) emissions from a variety of locations. BC deposition contributes to melting of glaciers and questions exist, of both scientific and policy interest, as to the origin of the BC reaching the glaciers. We use the adjoint of the GEOS-Chem model to identify the location from which BC arriving at a variety of locations in the Himalayas and Tibetan Plateau originates. We then calculate its direct and snow-albedo radiative forcing. We analyze the seasonal variation in the origin of BC using an adjoint sensitivity analysis, which provides a detailed map of the location of emissions that directly contribute to black carbon concentrations at receptor locations. We find that emissions from northern India and central China contribute the majority of BC to the Himalayas, although the precise location varies with season. The Tibetan Plateau receives most BC from western and central China, as well as from India, Nepal, the Middle East, Pakistan and other countries. The magnitude of contribution from each region varies with season and receptor location. We find that sources as varied as African biomass burning and Middle Eastern fossil fuel combustion can significantly contribute to the BC reaching the Himalayas and Tibetan Plateau. We compute radiative forcing in the snow-covered regions and find the forcing due to the BC induced snow-albedo effect to vary from 5-15 W m(-2) within the region, an order of magnitude larger than radiative forcing due to the direct effect, and with significant seasonal variation in the northern Tibetan Plateau. Radiative forcing from reduced snow albedo likely accelerates glacier melting. Our analysis may help inform mitigation efforts to slow the rate of glacial melt by identifying regions that make the largest contributions to BC deposition in the Himalayas and Tibetan Plateau.
引用
收藏
页码:2837 / 2852
页数:16
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