Effect of deposition temperature on ultra-low voltage resistive switching behavior of Fe-doped SrTiO3 films

被引:6
作者
Jiang, Xue [1 ]
Wei, Minglong [1 ]
Chan, Cheuk Ho [2 ]
Wang, Yingyue [1 ]
Lai, Ruilian [1 ]
Wang, Jianbo [1 ]
Dai, Jiyan [2 ]
Qiu, Xiaoyan [1 ]
机构
[1] Southwest Univ, Sch Phys Sci & Technol, Chongqing 400715, Peoples R China
[2] Hong Kong Polytech Univ, Dept Appl Phys, Hong Kong, Peoples R China
基金
中国国家自然科学基金;
关键词
THIN-FILMS; OXIDE; MECHANISMS; SURFACE;
D O I
10.1063/1.5123254
中图分类号
O59 [应用物理学];
学科分类号
摘要
The effect of deposition temperature on the microstructures and resistive switching properties of Fe-doped SrTiO3 (Fe-STO) films deposited via magnetron sputtering has been investigated. The as-deposited Fe-STO films change from amorphous to polycrystalline when the deposition temperature increases to 600 degrees C, but 800 degrees C-deposited Fe-STO films exhibit cracked surface morphologies with Sr-rich nanosheet segregation. Fe-STO films deposited at <= 600 degrees C exhibit reversible bipolar resistive switching behaviors with ultra-low switching voltages of <+/- 0.6V, while 450 degrees C-deposited Fe-STO films retain an ON/OFF resistance ratio of similar to 10(5) after more than 2500 endurance cycles and 600 degrees C-deposited Fe-STO films exhibit three different resistive switching patterns in sequence. Fe-assisted oxygen-vacancy conductive filaments are responsible for the ultra-low voltage resistive switching behaviors of Fe-STO films.
引用
收藏
页数:5
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共 43 条
[1]   Spectromicroscopic insights for rational design of redox-based memristive devices [J].
Baeumer, Christoph ;
Schmitz, Christoph ;
Ramadan, Amr H. H. ;
Du, Hongchu ;
Skaja, Katharina ;
Feyer, Vitaliy ;
Mueller, Philipp ;
Arndt, Benedikt ;
Jia, Chun-Lin ;
Mayer, Joachim ;
De Souza, Roger A. ;
Schneider, Claus Michael ;
Waser, Rainer ;
Dittmann, Regina .
NATURE COMMUNICATIONS, 2015, 6
[2]   Flexible nonvolatile resistive memory devices based on SrTiO3 nanosheets and polyvinylpyrrolidone composites [J].
Chen, Guilin ;
Zhang, Peng ;
Pan, Lulu ;
Qi, Lin ;
Yu, Fucheng ;
Gao, Cunxu .
JOURNAL OF MATERIALS CHEMISTRY C, 2017, 5 (37) :9799-9805
[3]   Comprehensive study of the resistance switching in SrTiO3 and Nb-doped SrTiO3 [J].
Chen, X. G. ;
Ma, X. B. ;
Yang, Y. B. ;
Chen, L. P. ;
Xiong, G. C. ;
Lian, G. J. ;
Yang, Y. C. ;
Yang, J. B. .
APPLIED PHYSICS LETTERS, 2011, 98 (12)
[4]   Structural characterisation of slightly Fe-doped SrTiO3 grown via a sol-gel hydrothermal synthesis [J].
Fuentes, S. ;
Munoz, P. ;
Barraza, N. ;
Chavez-Angel, E. ;
Sotomayor Torres, C. M. .
JOURNAL OF SOL-GEL SCIENCE AND TECHNOLOGY, 2015, 75 (03) :593-601
[5]   Roles of Schottky barrier and oxygen vacancies in the electroforming of SrTiO3 [J].
Guo, Xin .
APPLIED PHYSICS LETTERS, 2012, 101 (15)
[6]   Implementing ceramic materials into neuromorphic memory devices through oxide-based memristors [J].
Rutherford, Bethany X. .
AMERICAN CERAMIC SOCIETY BULLETIN, 2021, 100 (06) :48-48
[7]   Multilevel data storage memory based on polycrystalline SrTiO3 ultrathin film [J].
Hou, Pengfei ;
Gao, Zhanzhan ;
Ni, Kaikai .
RSC ADVANCES, 2017, 7 (78) :49753-49758
[8]   Memristor devices for neural networks [J].
Jeong, Hongsik ;
Shi, Luping .
JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2019, 52 (02)
[9]   Resistive states in strontium titanate thin films: Bias effects and mechanisms at high and low temperature [J].
Kubicek, M. ;
Taibl, S. ;
Navickas, E. ;
Hutter, H. ;
Fafilek, G. ;
Fleig, J. .
JOURNAL OF ELECTROCERAMICS, 2017, 39 (1-4) :197-209
[10]   Uncovering Two Competing Switching Mechanisms for Epitaxial and Ultrathin Strontium Titanate-Based Resistive Switching Bits [J].
Kubicek, Markus ;
Schmitt, Rafael ;
Messerschmitt, Felix ;
Rupp, Jennifer L. M. .
ACS NANO, 2015, 9 (11) :10737-10748