Recovery of uranium (VI) from aqueous solutions by the polyethyleneimine-functionalized reduced graphene oxide/molybdenum disulfide composition aerogels

被引:32
作者
Guo, Dongxuan [1 ]
Song, Xiumei [3 ]
Zhang, Lulu [1 ]
Chen, Weiwen [1 ]
Chu, Daiwei [1 ]
Tan, Lichao [1 ,2 ]
机构
[1] Harbin Univ Sci & Technol, Coll Chem & Environm Engn, Sch Mat Sci & Engn, Harbin 150040, Peoples R China
[2] Harbin Engn Univ, Minist Educ, Key Lab Superlight Mat & Surface Technol, Harbin 150001, Peoples R China
[3] Harbin Inst Technol, State Key Lab Urban Water Resource & Environm, Harbin 150090, Peoples R China
基金
中国博士后科学基金;
关键词
Uranium (VI); Adsorption; Polyethyleneimine; MoS2; Composition aerogels; METHYLENE-BLUE; ADSORPTION; SEAWATER; REMOVAL; EXTRACTION; NANOSHEETS; STRATEGY; GELATION; MWCNT; TIO2;
D O I
10.1016/j.jtice.2019.09.029
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
In this work, we have developed a facile route for the fabrication of polyethyleneimine-functionalized reduced graphene oxide/molybdenum disulfide composition aerogels (PEI-rGO/MoS2 CAs). The as-obtained nanomaterial (PEI-rGO/MoS2 CAs) is characterized by using scanning electron microscopy, transmission electron microscopy, Fourier-transform infrared spectroscopy, X-ray diffraction and X-ray photoelectron spectroscopy measurements. The different parameters regulating the adsorption of uranium (VI) such as contact time, pH and temperature are texted. The results show that the adsorption processes of uranium (VI) onto PEI-rGO/MoS2 CAs-3 are spontaneous and endothermic and well follow pseudo-second-order and Langmuir isotherm model. The equilibrium time and maximum adsorption capacity of PEI-rGO/MoS2 CAs-3 are 350 min and 184.53 mg g(-1). Therefore, PEI-rGO/MoS2 CAs holds the potential as promising adsorbent for the adsorption of uranium (VI). (C) 2019 Taiwan Institute of Chemical Engineers. Published by Elsevier B.V. All rights reserved.
引用
收藏
页码:198 / 205
页数:8
相关论文
共 37 条
[1]   Chemical and structural evaluation of activated carbon prepared from jute sticks for Brilliant Green dye removal from aqueous solution [J].
Asadullah, Mohammad ;
Asaduzzaman, Mohammad ;
Kabir, Mohammad Shajahan ;
Mostofa, Mohammad Golam ;
Miyazawa, Tomohisa .
JOURNAL OF HAZARDOUS MATERIALS, 2010, 174 (1-3) :437-443
[2]   On the Gelation of Graphene Oxide [J].
Bai, Hua ;
Li, Chun ;
Wang, Xiaolin ;
Shi, Gaoquan .
JOURNAL OF PHYSICAL CHEMISTRY C, 2011, 115 (13) :5545-5551
[3]   Supramolecular gels 'in action' [J].
Banerjee, Supratim ;
Das, Rajat K. ;
Maitra, Uday .
JOURNAL OF MATERIALS CHEMISTRY, 2009, 19 (37) :6649-6687
[4]   Adsorption of semisoft pollutants onto Bi2S3/Ag2S-AC under the influence of ultrasonic waves as external filed [J].
Dashtian, Kheibar ;
Porhemat, Sima ;
Rezvani, Ali Reza ;
Ghaedi, Mehrorang ;
Sabzehmeidani, Mohammad Mehdi .
JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY, 2018, 60 :390-400
[5]   Sorption of U(VI) on magnetic illite: effects of pH, ions, humic substances and temperature [J].
Du, Yaofang ;
Yin, Zhuoxin ;
Wu, Hanyu ;
Li, Ping ;
Qi, Wei ;
Wu, Wangsuo .
JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY, 2015, 304 (02) :793-804
[6]  
Gu Z, 2014, J RADIOANAL NUCL CHE
[7]   Amidoxime-modified mesoporous silica for uranium adsorption under seawater conditions [J].
Gunathilake, Chamila ;
Gorka, Joanna ;
Dai, Shen ;
Jaroniec, Mietek .
JOURNAL OF MATERIALS CHEMISTRY A, 2015, 3 (21) :11650-11659
[8]   Freestanding hierarchical nickel molybdate@reduced graphene oxide@nickel aluminum layered double hydroxides nanoarrays assembled from well-aligned uniform nanosheets as binder-free electrode materials for high performance supercapacitors [J].
Guo, Dongxuan ;
Song, Xiumei ;
Li, Bonan ;
Tan, Lichao ;
Ma, Huiyuan ;
Pang, Haijun ;
Wang, Xinming ;
Zhang, Lulu .
JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2019, 544 :46-52
[9]   A facile dissolved and reassembled strategy towards sandwich-like rGO@NiCoAl-LDHs with excellent supercapacitor performance [J].
Guo, Dongxuan ;
Song, Xiumei ;
Tan, Lichao ;
Ma, Huiyuan ;
Sun, Weifeng ;
Pang, Haijun ;
Zhang, Lulu ;
Wang, Xinming .
CHEMICAL ENGINEERING JOURNAL, 2019, 356 :955-963
[10]   Removal of UO22+ from aqueous solution using halloysite nanotube-Fe3O4 composite [J].
He, Wenfang ;
Chen, Yuantao ;
Zhang, Wei ;
Hu, Chunlian ;
Wang, Jian ;
Wang, Pingping .
KOREAN JOURNAL OF CHEMICAL ENGINEERING, 2016, 33 (01) :170-177