Charge Fluctuations on a Flat Interface between Dielectric and Electrolyte or Dense Plasma

被引:0
|
作者
Rosenfeld, E., V [1 ]
Zakharov, A., V [2 ]
Djakin, V. V. [1 ]
机构
[1] Ural Branch Russian Acad Sci, Inst Met Phys, Ekaterinburg 620990, Russia
[2] Russian Acad Sci, Space Res Inst, Moscow 117997, Russia
关键词
DUST GRAIN; PARTICLES;
D O I
10.1021/acs.langmuir.2c01347
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
An interface between a dielectric and a medium containing charge carriers with moderate mobility is considered. In equilibrium, stochastic fluxes of positive and negative particles toward the surface have equal average current density j(0), and we suppose that the surface absorbs all falling charges. All over the surface, this results in the emergence of oppositely charged spots of various sizes D fluctuating and interacting with each other. Fourier expansion reduces this collection of interacting spots to the ensemble of independently fluctuating charge density waves. An exact solution of the Poisson equation for a single wave on a flat surface was obtained and provided strict proof that a fluctuating electric field is quite strong just above each charge spot but diminishes exponentially with the distance from the plane. The lifetime tau of a charge spot is inversely proportional to the density j(0) of the stochastic current while proportional to j(0) fluctuation's amplitudes independent of j(0)tau. The fluctuation's parameter dependence on the charge spot's size D can vary according to the conducting medium properties.
引用
收藏
页码:9382 / 9388
页数:7
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