Photogating of mono- and few-layer MoS2

被引:93
作者
Miller, Bastian [1 ,2 ,3 ]
Parzinger, Eric [1 ,2 ,3 ]
Vernickel, Anna [1 ,2 ,3 ]
Holleitner, Alexander W. [1 ,2 ,3 ]
Wurstbauer, Ursula [1 ,2 ,3 ]
机构
[1] Tech Univ Munich, Walter Schottky Inst, D-85748 Garching, Germany
[2] Tech Univ Munich, Dept Phys, D-85748 Garching, Germany
[3] NIM, D-80799 Munich, Germany
关键词
MONOLAYER MOS2; PHOTOLUMINESCENCE; RAMAN; EMISSION; GRAPHENE;
D O I
10.1063/1.4916517
中图分类号
O59 [应用物理学];
学科分类号
摘要
We describe a photogating effect in mono- and few-layer MoS2, which allows the control of the charge carrier density by almost two orders of magnitude without electrical contacts. Our Raman studies are consistent with physisorbed environmental molecules, which effectively deplete the intrinsically n-doped charge carrier system via charge transfer and which can be gradually removed by the exposure to light. This photogating process is reversible and precisely tunable by the light intensity. The photogating efficiency is quantified by comparison with measurements on electrostatically gated MoS2. (C) 2015 AIP Publishing LLC.
引用
收藏
页数:4
相关论文
共 25 条
[1]   Extraordinary Sunlight Absorption and One Nanometer Thick Photovoltaics Using Two-Dimensional Monolayer Materials [J].
Bernardi, Marco ;
Palummo, Maurizia ;
Grossman, Jeffrey C. .
NANO LETTERS, 2013, 13 (08) :3664-3670
[2]   The effect of the substrate on the Raman and photoluminescence emission of single-layer MoS2 [J].
Buscema, Michele ;
Steele, Gary A. ;
van der Zant, Herre S. J. ;
Castellanos-Gomez, Andres .
NANO RESEARCH, 2014, 7 (04) :561-571
[3]   Symmetry-dependent phonon renormalization in monolayer MoS2 transistor [J].
Chakraborty, Biswanath ;
Bera, Achintya ;
Muthu, D. V. S. ;
Bhowmick, Somnath ;
Waghmare, U. V. ;
Sood, A. K. .
PHYSICAL REVIEW B, 2012, 85 (16)
[4]   Bandgap Engineering of Strained Monolayer and Bilayer MoS2 [J].
Conley, Hiram J. ;
Wang, Bin ;
Ziegler, Jed I. ;
Haglund, Richard F., Jr. ;
Pantelides, Sokrates T. ;
Bolotin, Kirill I. .
NANO LETTERS, 2013, 13 (08) :3626-3630
[5]   Monitoring dopants by Raman scattering in an electrochemically top-gated graphene transistor [J].
Das, A. ;
Pisana, S. ;
Chakraborty, B. ;
Piscanec, S. ;
Saha, S. K. ;
Waghmare, U. V. ;
Novoselov, K. S. ;
Krishnamurthy, H. R. ;
Geim, A. K. ;
Ferrari, A. C. ;
Sood, A. K. .
NATURE NANOTECHNOLOGY, 2008, 3 (04) :210-215
[6]   Temperature-dependent phonon shifts in monolayer MoS2 [J].
Lanzillo, Nicholas A. ;
Birdwell, A. Glen ;
Amani, Matin ;
Crowne, Frank J. ;
Shah, Pankaj B. ;
Najmaei, Sina ;
Liu, Zheng ;
Ajayan, Pulickel M. ;
Lou, Jun ;
Dubey, Madan ;
Nayak, Saroj K. ;
O'Regan, Terrance P. .
APPLIED PHYSICS LETTERS, 2013, 103 (09)
[7]   Sensing Behavior of Atomically Thin-Layered MoS2 Transistors [J].
Late, Dattatray J. ;
Huang, Yi-Kai ;
Liu, Bin ;
Acharya, Jagaran ;
Shirodkar, Sharmila N. ;
Luo, Jiajun ;
Yan, Aiming ;
Charles, Daniel ;
Waghmare, Umesh V. ;
Dravid, Vinayak P. ;
Rao, C. N. R. .
ACS NANO, 2013, 7 (06) :4879-4891
[8]   Anomalous Lattice Vibrations of Single- and Few-Layer MoS2 [J].
Lee, Changgu ;
Yan, Hugen ;
Brus, Louis E. ;
Heinz, Tony F. ;
Hone, James ;
Ryu, Sunmin .
ACS NANO, 2010, 4 (05) :2695-2700
[9]   Carrier Control of MoS2 Nanoflakes by Functional Self-Assembled Monolayers [J].
Li, Yang ;
Xu, Cheng-Yan ;
Hu, PingAn ;
Zhen, Liang .
ACS NANO, 2013, 7 (09) :7795-7804
[10]  
Lopez-Sanchez O, 2013, NAT NANOTECHNOL, V8, P497, DOI [10.1038/NNANO.2013.100, 10.1038/nnano.2013.100]