Saturated absorption spectroscopy of buffer-gas-cooled Barium monofluoride molecules

被引:14
作者
Bu, Wenhao
Zhang, Yuhe
Liang, Qian
Chen, Tao
Yan, Bo [1 ]
机构
[1] Zhejiang Univ, Interdisciplinary Ctr Quantum Informat, State Key Lab Modern Opt Instrumentat, Hangzhou 310027, Peoples R China
基金
中国国家自然科学基金;
关键词
cold molecule; saturated spectroscopy; buffer gas cooling; BaF; HYPERFINE-STRUCTURE; COLD; ATOMS; BEAM;
D O I
10.1007/s11467-022-1194-x
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We report an experimental investigation on the Doppler-free saturated absorption spectroscopy of buffer-gas-cooled Barium monofluoride (BaF) molecules in a 4 K cryogenic cell. The obtained spectra with a resolution of 19 MHz, much smaller than previously observed in absorption spectroscopy, clearly resolve the hyperfine transitions. Moreover, we use these high-resolution spectra to fit the hyperfine splittings of excited A(v = 0) state and find the hyperfine splitting of the laser-cooling-relevant A(2)Pi(1/2)(v= 0, J = 1/2,+) state is about 18 MHz, much higher than the previous theoreti- cally predicted value. This provides important missing information for laser cooling of BaF molecules.
引用
收藏
页数:7
相关论文
共 63 条
[1]   Measuring the electric dipole moment of the electron in BaF [J].
Aggarwal, Parul ;
Bethlem, Hendrick L. ;
Borschevsky, Anastasia ;
Denis, Malika ;
Esajas, Kevin ;
Haase, Pi A. B. ;
Hao, Yongliang ;
Hoekstra, Steven ;
Jungmann, Klaus ;
Meijknecht, Thomas B. ;
Mooij, Maarten C. ;
Timmermans, Rob G. E. ;
Ubachs, Wim ;
Willmann, Lorenz ;
Zapara, Artem .
EUROPEAN PHYSICAL JOURNAL D, 2018, 72 (11)
[2]   Buffer-gas cooling, high-resolution spectroscopy, and optical cycling of barium monofluoride molecules [J].
Albrecht, Ralf ;
Scharwaechter, Michael ;
Sixt, Tobias ;
Hofer, Lucas ;
Langen, Tim .
PHYSICAL REVIEW A, 2020, 101 (01)
[3]   Demonstration of a Sensitive Method to Measure Nuclear-Spin-Dependent Parity Violation [J].
Altuntas, Emine ;
Ammon, Jeffrey ;
Cahn, Sidney B. ;
DeMille, David .
PHYSICAL REVIEW LETTERS, 2018, 120 (14)
[4]   An optical tweezer array of ultracold molecules [J].
Anderegg, Loic ;
Cheuk, Lawrence W. ;
Bao, Yicheng ;
Burchesky, Sean ;
Ketterle, Wolfgang ;
Ni, Kang-Kuen ;
Doyle, John M. .
SCIENCE, 2019, 365 (6458) :1156-+
[5]   Laser cooling of optically trapped molecules [J].
Anderegg, Loic ;
Augenbraun, Benjamin L. ;
Bao, Yicheng ;
Burchesky, Sean ;
Cheuk, Lawrence W. ;
Ketterle, Wolfgang ;
Doyle, John M. .
NATURE PHYSICS, 2018, 14 (09) :890-893
[6]   Radio Frequency Magneto-Optical Trapping of CaF with High Density [J].
Anderegg, Loic ;
Augenbraun, Benjamin L. ;
Chae, Eunmi ;
Hemmerling, Boerge ;
Hutzler, Nicholas R. ;
Ravi, Aakash ;
Collopy, Alejandra ;
Ye, Jun ;
Ketterle, Wolfgang ;
Doyle, John M. .
PHYSICAL REVIEW LETTERS, 2017, 119 (10)
[7]   A coherent all-electrical interface between polar molecules and mesoscopic superconducting resonators [J].
Andre, A. ;
Demille, D. ;
Doyle, J. M. ;
Lukin, M. D. ;
Maxwell, S. E. ;
Rabl, P. ;
Schoelkopf, R. J. ;
Zoller, P. .
NATURE PHYSICS, 2006, 2 (09) :636-642
[8]   Laser-cooled polyatomic molecules for improved electron electric dipole moment searches [J].
Augenbraun, Benjamin L. ;
Lasner, Zack D. ;
Frenett, Alexander ;
Sawaoka, Hiromitsu ;
Miller, Calder ;
Steimle, Timothy C. ;
Doyle, John M. .
NEW JOURNAL OF PHYSICS, 2020, 22 (02)
[9]   Magneto-optical trapping of a diatomic molecule [J].
Barry, J. F. ;
McCarron, D. J. ;
Norrgard, E. B. ;
Steinecker, M. H. ;
DeMille, D. .
NATURE, 2014, 512 (7514) :286-+
[10]   A bright, slow cryogenic molecular beam source for free radicals [J].
Barry, J. F. ;
Shuman, E. S. ;
DeMille, D. .
PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2011, 13 (42) :18936-18947