Formation mechanism and optical properties of nanocrystalline silicon in silicon oxide

被引:11
作者
Kim, JH [1 ]
Jeon, KA [1 ]
Lee, SY [1 ]
机构
[1] Yonsei Univ, Dept Elect & Elect Engn, Seoul 120749, South Korea
关键词
D O I
10.1063/1.1935136
中图分类号
O59 [应用物理学];
学科分类号
摘要
Silicon nanocrystals with diameters ranging from 1.5 to 3 nm were formed on silicon substrates by using a pulsed laser deposition (PLD) followed by annealing and oxidation. The optical and structural properties of the films have been investigated as a function of deposition temperature, annealing, and oxidation process. When the deposition temperature increased, photoluminescence intensity abruptly decreased and peaks showed redshift. Annealing process can reduce the number of defect centers. Oxidation has considerable effect upon the formation and isolation of the nanocrystals. These results suggest that the formation mechanism of Si nanocrystals by using PLD could be explained by three steps of growth, passivating defect centers, and isolation, sequentially. (c) 2005 American Institute of Physics.
引用
收藏
页数:4
相关论文
共 21 条
[1]   High-density crystalline quantum dots in blue emitting porous silicon [J].
Chen, QW ;
Li, XJ ;
Zhou, GE ;
Zhu, JS ;
Zhang, SY ;
Jia, YB .
JOURNAL OF APPLIED PHYSICS, 1997, 81 (12) :7970-7972
[2]   The effect of ion-irradiation and annealing on the luminescence of Si nanocrystals in SiO2 [J].
Cheylan, S ;
Langford, N ;
Elliman, RG .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 2000, 166 :851-856
[3]   Si-rich/SiO2 nanostructured multilayers by reactive magnetron sputtering [J].
Gourbilleau, F ;
Portier, X ;
Ternon, C ;
Voivenel, P ;
Madelon, R ;
Rizk, R .
APPLIED PHYSICS LETTERS, 2001, 78 (20) :3058-3060
[4]   Annealing effect on the photoluminescence of Si nanocrystallites thin films [J].
Jeon, KA ;
Kim, JH ;
Choi, JB ;
Han, KB ;
Lee, SY .
MATERIALS SCIENCE & ENGINEERING C-BIOMIMETIC AND SUPRAMOLECULAR SYSTEMS, 2003, 23 (6-8) :1017-1019
[5]   Surface modification of laser ablated YBCO target [J].
Jeong, YS ;
Lee, SY ;
Jang, HK ;
Yang, IS ;
Moon, SH ;
Oh, B .
APPLIED SURFACE SCIENCE, 1997, 109 :424-427
[6]   Temperature effects on the formation of Si nanoclusters [J].
Kim, JH ;
Jeon, KA ;
Lee, SY .
APPLIED SURFACE SCIENCE, 2004, 226 (1-3) :68-71
[7]  
Kim JH, 2002, J KOREAN PHYS SOC, V41, P514
[8]   High temperature deformation behavior of a γ TiAl alloy determined using the load-relaxation test [J].
Kim, JH ;
Shin, DH ;
Semiatin, SL ;
Lee, CS .
MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING, 2003, 344 (1-2) :146-157
[9]   Laser wavelength effect on the light emission properties of nanocrystalline Si on Si substrate fabricated by pulsed laser deposition [J].
Kim, JH ;
Jeon, KA ;
Shim, ES ;
Lee, SY .
MATERIALS SCIENCE AND ENGINEERING B-SOLID STATE MATERIALS FOR ADVANCED TECHNOLOGY, 2002, 89 (1-3) :70-72
[10]   Effect of passivation and aging on the photoluminescence of silicon nanocrystals [J].
Ledoux, G ;
Gong, J ;
Huisken, F .
APPLIED PHYSICS LETTERS, 2001, 79 (24) :4028-4030