Engaging nanoporous carbons in "beyond adsorption" applications: Characterization, challenges and performance

被引:46
作者
Ania, Conchi O. [1 ]
Armstrong, Phillip A. [2 ]
Bandosz, Teresa J. [3 ]
Beguin, Francois [4 ]
Carvalho, Ana P. [5 ]
Celzard, Alain [6 ]
Frackowiak, Elzbieta [4 ]
Gilarranz, Miguel A. [7 ]
Laszlo, Krisztina [8 ]
Matos, Juan [9 ]
Pereira, M. Fernando R. [10 ]
机构
[1] Univ Orleans, CNRS, CEMHTI, UPR 3079, F-45071 Orleans, France
[2] Morgan Adv Mat, 310 Innovat Blvd,Suite 250, State Coll, PA 16803 USA
[3] CUNY City Coll, Dept Chem & Biochem, 160 Convent Ave, New York, NY 10031 USA
[4] Poznan Univ Tech, Inst Chem & Tech Electrochem, Berdychowo 4, PL-60965 Poznan, Poland
[5] Univ Lisbon, Fac Ciencias, Dept Quim & Bioquim, Ctr Quim Estrutural Polo Ciencias, P-1749016 Lisbon, Portugal
[6] Univ Lorraine, IJL, CNRS, F-88000 Epinal, France
[7] Univ Autonoma Madrid, Dept Chem Engn, Madrid 28049, Spain
[8] Budapest Univ Technol & Econ, Dept Phys Chem & Mat Sci, H-1521 Budapest, Hungary
[9] Univ Autonoma Chile, Fac Ingn, Inst Ciencias Quim Aplicadas, Santiago 8900000, Chile
[10] Univ Porto, Fac Engn, Lab Catalysis & Mat LSRE LCM, Lab Separat & React Engn, P-4200465 Porto, Portugal
基金
欧盟地平线“2020”;
关键词
Nanoporous carbons; Characterization; Energy storage; Catalysis; Surface chemistry; Defects; OXYGEN REDUCTION REACTION; WASTE-WATER TREATMENT; RELATIVE PHOTONIC EFFICIENCIES; METAL-FREE ELECTROCATALYST; ACTIVE SURFACE-AREA; PHOTOCATALYTIC DEGRADATION; OXIDATIVE DEHYDROGENATION; RAMAN-SPECTROSCOPY; SUSPENDED MIXTURE; HETEROGENEOUS PHOTOCATALYSIS;
D O I
10.1016/j.carbon.2020.03.056
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
This paper addresses the challenges of explaining the behavior of porous carbons in cutting-edge applications related to energy storage, catalysis, photocatalysis, and advanced separation based on reactive adsorption. It is a summary of the outcomes of the extensive discussion which took place during the workshop "Beyond Adsorption-II: new perspectives and challenges for nanoporous carbons," organized as a satellite event to the International Carbon Conference on July 20th, 2019 in New York. It is not our intention to provide a tutorial on the applications, characterization or performance testing of porous carbons; we would rather like to focus on the controversy of the results and phenomena, on the explanation of findings, and on raising concerns to the growing carbon-researching scientific community about the importance of understanding the features of nanoporous carbons by choosing an appropriate characterization technique that will bring meaningful information. We want to emphasize that nanoporous carbons have unique features ensuring them making a marked advance in science and technology. Even though recent studies have shown their potential in various emerging applications, the origin of such performance is not yet well understood. Thus, scientists are encouraged to focus on a precise characterization of porous carbons using a set of complementary techniques for triggering future technological developments. (C) 2020 Elsevier Ltd. All rights reserved.
引用
收藏
页码:69 / 84
页数:16
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