Ultrahigh Carrier Mobilities in Ferroelectric Domain Wall Corbino Cones at Room Temperature

被引:15
作者
McCluskey, Conor J. [1 ]
Colbear, Matthew G. [1 ]
McConville, James P., V [1 ]
McCartan, Shane J. [1 ]
Maguire, Jesi R. [1 ]
Conroy, Michele [2 ,3 ]
Moore, Kalani [2 ,3 ]
Harvey, Alan [2 ,3 ]
Trier, Felix [4 ,5 ]
Bangert, Ursel [2 ,3 ]
Gruverman, Alexei [6 ]
Bibes, Manuel [4 ]
Kumar, Amit [1 ]
McQuaid, Raymond G. P. [1 ]
Gregg, J. Marty [1 ]
机构
[1] Queens Univ Belfast, Sch Math & Phys, Belfast BT7 1NN, Antrim, North Ireland
[2] Univ Limerick, Dept Phys, Limerick V94 T9PX, Ireland
[3] Univ Limerick, Bernal Inst, Limerick V94 T9PX, Ireland
[4] Univ Paris Saclay, CNRS, Thales, Unite Mixte Phys, F-91767 Palaiseau, France
[5] Tech Univ Denmark, Dept Energy Convers & Storage, DK-2800 Lyngby, Denmark
[6] Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA
基金
英国工程与自然科学研究理事会;
关键词
carrier mobility; Corbino disks; domain walls; ferroelectrics; magnetoresistance; ELECTRON-GAS; MAGNETORESISTANCE; NIOBATE; SUPERCONDUCTIVITY; CONDUCTIVITY; CONDUCTANCE; MEMORY; DISK;
D O I
10.1002/adma.202204298
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Recently, electrically conducting heterointerfaces between dissimilar band insulators (such as lanthanum aluminate and strontium titanate) have attracted considerable research interest. Charge transport and fundamental aspects of conduction have been thoroughly explored. Perhaps surprisingly, similar studies on conceptually much simpler conducting homointerfaces, such as domain walls, are not nearly so well developed. Addressing this disparity, magnetoresistance is herein reported in approximately conical 180 degrees charged domain walls, in partially switched ferroelectric thin-film single-crystal lithium niobate. This system is ideal for such measurements: first, the conductivity difference between domains and domain walls is unusually large (a factor of 10(13)) and hence currents driven through the thin film, between planar top and bottom electrodes, are overwhelmingly channeled along the walls; second, when electrical contact is made to the top and bottom of the domain walls and a magnetic field is applied along their cone axes, then the test geometry mirrors that of a Corbino disk: a textbook arrangement for geometric magnetoresistance measurement. Data imply carriers with extremely high room-temperature Hall mobilities of up to approximate to 3700 cm(2) V-1 s(-1). This is an unparalleled value for oxide interfaces (and for bulk oxides) comparable to mobilities in other systems seen at cryogenic, rather than at room, temperature.
引用
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页数:10
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