Visible light degradation and separation of RhB by magnetic Fe3O4/ZnO/g-C3N4 nanoparticles

被引:18
作者
Wang, Yue [1 ]
Li, Xuefei [1 ]
Yang, Yuzhe [1 ]
Yang, Jinghai [1 ]
Zhang, Nan [1 ]
Wu, Xingtong [2 ]
Li, Xiuyan [1 ]
机构
[1] Jilin Normal Univ, Key Lab Funct Mat Phys & Chem, Minist Educ, Changchun 136000, Peoples R China
[2] Jiangxi Agr Univ, Sch Engn, Nanchang 330045, Jiangxi, Peoples R China
关键词
ENHANCED PHOTOCATALYTIC PERFORMANCE; CARBON NITRIDE NANOSHEETS; HIGHLY EFFICIENT; G-C3N4; TIO2; ZNO; COMPOSITE; CATALYST; FABRICATION; INTERFACE;
D O I
10.1007/s10854-020-03078-3
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
Photocatalytic technology has the potential to eliminate organic pollutants in wastewater. Herein, superparamagnetic Fe3O4/ZnO/g-C3N4 composite photocatalysts are reported. Photocatalysts with different g-C3N4 concentrations were prepared and their photocatalytic activities were tested. The composite samples have better photocatalytic activity in visible light. This result suggests that the heterogeneous junction of the composite photocatalyst retards carrier recombination: because of the presence of g-C3N4 nanosheets, the optical response range of photocatalyst is expanded. The introduction of Fe3O4 nanoparticles can solve the problem of difficult recovery of powder photocatalyst. Photocatalyst activity only slightly decreases after three cycles of use.
引用
收藏
页码:5187 / 5197
页数:11
相关论文
共 55 条
[1]   Photocatalytic Activity Enhanced via g-C3N4 Nanoplates to Nanorods [J].
Bai, Xiaojuan ;
Wang, Li ;
Zong, Ruilong ;
Zhu, Yongfa .
JOURNAL OF PHYSICAL CHEMISTRY C, 2013, 117 (19) :9952-9961
[2]   Magnetic Fe@g-C3N4: A Photoactive Catalyst for the Hydrogenation of Alkenes and Alkynes [J].
Baig, R. B. Nasir ;
Verma, Sanny ;
Varma, Rajender S. ;
Nadagouda, Mallikarjuna N. .
ACS SUSTAINABLE CHEMISTRY & ENGINEERING, 2016, 4 (03) :1661-1664
[3]   Spatial engineering of photo-active sites on g-C3N4 for efficient solar hydrogen generation [J].
Chen, Jie ;
Shen, Shaohua ;
Guo, Penghui ;
Wu, Po ;
Guo, Liejin .
JOURNAL OF MATERIALS CHEMISTRY A, 2014, 2 (13) :4605-4612
[4]   Multiphase TiO2 surface coating g-C3N4 formed a sea urchin like structure with interface effects and improved visible-light photocatalytic performance for the degradation of ibuprofen [J].
Chen, Xi ;
Li, Xuefei ;
Yang, Jinghai ;
Sun, Qianyu ;
Yang, Yuzhe ;
Wu, Xingtong .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2018, 43 (29) :13284-13293
[5]   Preparation of sphere-like g-C3N4/BiOI photocatalysts via a reactable ionic liquid for visible-light-driven photocatalytic degradation of pollutants [J].
Di, Jun ;
Xia, Jiexiang ;
Yin, Sheng ;
Xu, Hui ;
Xu, Li ;
Xu, Yuanguo ;
He, Minqiang ;
Li, Huaming .
JOURNAL OF MATERIALS CHEMISTRY A, 2014, 2 (15) :5340-5351
[6]   Efficient synthesis of polymeric g-C3N4 layered materials as novel efficient visible light driven photocatalysts [J].
Dong, Fan ;
Wu, Liwen ;
Sun, Yanjuan ;
Fu, Min ;
Wu, Zhongbiao ;
Lee, S. C. .
JOURNAL OF MATERIALS CHEMISTRY, 2011, 21 (39) :15171-15174
[7]   ENVIRONMENTAL APPLICATIONS OF SEMICONDUCTOR PHOTOCATALYSIS [J].
HOFFMANN, MR ;
MARTIN, ST ;
CHOI, WY ;
BAHNEMANN, DW .
CHEMICAL REVIEWS, 1995, 95 (01) :69-96
[8]   High saturation magnetization Fe3O4 nanoparticles prepared by one-step reduction method in autoclave [J].
Hu, Ping ;
Kang, Lu ;
Chang, Tian ;
Yang, Fan ;
Wang, Hua ;
Zhang, Yang ;
Yang, Jun ;
Wang, Kuai-she ;
Du, Jinjing ;
Yang, Zhanlin .
JOURNAL OF ALLOYS AND COMPOUNDS, 2017, 728 :88-92
[9]   Effect of contact interface between TiO2 and g-C3N4 on the photoreactivity of g-C3N4/TiO2 photocatalyst: (001) vs (101) facets of TiO2 [J].
Huang, Ze'ai ;
Sun, Qiong ;
Lv, Kangle ;
Zhang, Zehui ;
Li, Mei ;
Li, Bing .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2015, 164 :420-427
[10]   Highly efficient heterojunction photocatalyst based on nanoporous g-C3N4 sheets modified by Ag3PO4 nanoparticles: Synthesis and enhanced photocatalytic activity [J].
Jiang, Deli ;
Zhu, Jianjun ;
Chen, Min ;
Xie, Jimin .
JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2014, 417 :115-120