Bismuth activated succulent-like binary metal sulfide heterostructure as a binder-free electrocatalyst for enhanced oxygen evolution reaction

被引:36
作者
Wang, Shuai [1 ]
Xue, Weidong [1 ]
Fang, Yuan [1 ]
Li, Yongqing [2 ]
Yan, Liuliu [2 ]
Wang, Wenjian [1 ]
Zhao, Rui [1 ]
机构
[1] Univ Elect Sci & Technol China, Sch Mat & Energy, 4,Sect 2,North Jianshe Rd, Chengdu 610054, Peoples R China
[2] Naval Univ Engn, Coll Naval Architecture & Ocean Engn, 717 Jiefang Ave, Wuhan 430033, Peoples R China
关键词
Oxygen evolution reaction; Bi2S3/Ni3S2/NF; Electronic inductive effect; Self-assembled; Heterostructure; HIGHLY EFFICIENT; NANOWIRE ARRAYS; NICKEL FOAM; NI FOAM; WATER; NANOPARTICLES; NANOSHEETS; PERFORMANCE; NICO2S4;
D O I
10.1016/j.jcis.2020.03.098
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Oxygen evolution reaction (OER) is the key to achieve highly efficient hydrogen production during water splitting. Herein, flexible nanorods-integrated succulent-like Bi2S3/Ni3S2/NF heterostructure has been prepared by a facile solvothermal method and applied for OER. We highlight the unique nonequivalent sp a hybridization of P-region metal based sulfides, which makes a possibility of electronic inductive effect and enhanced electrocatalytic performance. The Bi2S3/Ni3S2/NF catalyst shows low overpotential 268 mV at 10 mA cm(-2) and low Tafel slope of 82 mV dec(-1). Long-term stability evaluated at high current density suggests that succulent-like Bi2S3/Ni3S2 could be a promising alternative to noble-metal based electrocatalysts for water oxidation reaction in alkaline medium. (C) 2020 Elsevier Inc. All rights reserved.
引用
收藏
页码:150 / 157
页数:8
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