Photoluminescence properties of the entire excitonic series in Cu2O

被引:38
作者
Takahata, Mitsuyoshi [1 ]
Naka, Nobuko [1 ]
机构
[1] Kyoto Univ, Dept Phys, Sakyo Ku, Kitashirakawa Oiwake Cho, Kyoto 6068502, Japan
关键词
RAMAN-SCATTERING; CUPROUS-OXIDE; ABSORPTION; RECOMBINATION; LUMINESCENCE; EXCITATION; DYNAMICS; DECAY;
D O I
10.1103/PhysRevB.98.195205
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We investigated the photoluminescence spectra of Cu2O under photoexcitation at 3.05 eV across the violet band gap. The following three features were found: photoluminescence from blue and violet excitons; photoluminescence from yellow excitons of s, d, and f states in addition to p states with a quantum number up to ten; and emissions associated with the inelastic collision of the is yellow excitons. The first process is relevant for the separation of radiative and nonradiative decay rates. The second process likely indicates radiative enhancement of high Rydberg yellow excitons. The last process verifies up-conversion of 1s yellow paraexcitons into higher Rydberg states, which is a critical factor impeding the realization of a high-density paraexciton gas towards transition to the Bose-Einstein condensation.
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页数:10
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共 53 条
[1]   Magneto-absorption spectra of hydrogen-like yellow exciton series in cuprous oxide: excitons in strong magnetic fields [J].
Artyukhin, Sergey ;
Fishman, Dmitry ;
Faugeras, Clement ;
Potemski, Marek ;
Revcolevschi, Alexandre ;
Mostovoy, Maxim ;
van Loosdrecht, Paul H. M. .
SCIENTIFIC REPORTS, 2018, 8
[2]  
Assmann M, 2016, NAT MATER, V15, P741, DOI [10.1038/nmat4622, 10.1038/NMAT4622]
[3]   Theory of the lifetime of an exciton incoherently created below its resonance frequency by inelastic scattering [J].
Bamba, Motoaki ;
Wakaiki, Shuji ;
Ichida, Hideki ;
Mizoguchi, Kohji ;
Kim, DaeGwi ;
Nakayama, Masaaki ;
Kanematsu, Yasuo .
PHYSICAL REVIEW B, 2015, 91 (23)
[4]   STUDY OF PHONON DISPERSION-RELATIONS IN CUPROUS-OXIDE BY INELASTIC NEUTRON-SCATTERING [J].
BEG, MM ;
SHAPIRO, SM .
PHYSICAL REVIEW B, 1976, 13 (04) :1728-1734
[5]   INTRINSIC ABSORPTION AND REFLECTION OF CUPROUS OXIDE IN THE 2.5 TO 6.5 eV REGION [J].
Brahms, S. ;
Nikitine, S. .
SOLID STATE COMMUNICATIONS, 1965, 3 (08) :209-212
[6]   RIGID ION MODEL LATTICE DYNAMICS OF CUPRITE (CU2O) [J].
CARABATOS, C ;
PREVOT, B .
PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS, 1971, 44 (02) :701-+
[7]   Optoelectronic properties of ZnSe/ZnMgSSe multiple quantum wells [J].
Chang, CW ;
Yang, HC ;
Chen, CH ;
Chang, HJ ;
Chen, YF .
JOURNAL OF APPLIED PHYSICS, 2001, 89 (07) :3725-3729
[8]   Intra-excitonic relaxation dynamics in ZnO [J].
Chernikov, Alexej ;
Koch, Martin ;
Laumer, Bernhard ;
Wassner, Thomas A. ;
Eickhoff, Martin ;
Koch, Stephan W. ;
Chatterjee, Sangam .
APPLIED PHYSICS LETTERS, 2011, 99 (23)
[9]   RAMAN-SCATTERING, LUMINESCENCE, AND EXCITON-PHONON COUPLING IN CU2O [J].
COMPAAN, A ;
CUMMINS, HZ .
PHYSICAL REVIEW B, 1972, 6 (12) :4753-4757
[10]   ETUDE SPECTROPHOTOMETRIQUE DE LABSORPTION BLEUE ET VIOLETTE DE CU2O [J].
DAUNOIS, A ;
DEISS, JL ;
MEYER, B .
JOURNAL DE PHYSIQUE, 1966, 27 (3-4) :142-&