Nitrite sensing based on the carbon dots-enhanced chemiluminescence from peroxynitrous acid and carbonate

被引：85

作者：

Lin, Zhen ^{[1
,2
]}

Dou, Xiangnan ^{[2
]}

Li, Haifang ^{[2
]}

Ma, Yuan ^{[2
]}

Lin, Jin-Ming ^{[2
]}

机构：

[1] Fujian Med Univ, Fac Pharm, Dept Pharmaceut Anal, Fuzhou 350004, Peoples R China

[2] Tsinghua Univ, Dept Chem, Beijing Key Lab Microanalyt Methods & Instrumenta, Beijing 100084, Peoples R China

来源：

TALANTA | 2015年 / 132卷

基金：

中国国家自然科学基金;

关键词：

Chemiluminescence; Carbon dots; Peroxynitrous acid; Carbonate; QUANTUM DOTS; OXIDE; ION; TRYPTOPHAN; CO2;

D O I：

10.1016/j.talanta.2014.09.046

中图分类号：

O65 [分析化学];

学科分类号：

070302 ; 081704 ;

摘要：

In this work, chemiluminescence (CL) from peroxynitrous acid (ONOOH)-carbonate system greatly amplified by carbon dots was observed. The CL mechanism of the ONOOH-carbonate-carbon dots system has been investigated and the results reveal that the carbon dots could serve as the energy acceptor, which gives us new insight into the optical properties of the new emerging carbon nanomaterial. There is a good linear relationship between the CL signal and the concentration of the nitrite using for ONOOH formation, which provides us a nitrite sensing method with sensitivity as high as 5.0 x 10(-9) M (S/N= 3). The method has been successfully applied to the determination of nitrite in tap water with the recovery of 98%. The standard deviations are within 2.5%. (C) 2014 Elsevier B.V. All rights reserved.

引用

页码：457 / 462

页数：6

共 37 条

[1] Peroxynitrite-dependent tryptophan nitration [J].

Alvarez, B ;

Rubbo, H ;

Kirk, M ;

Barnes, S ;

Freeman, BA ;

Radi, R .

CHEMICAL RESEARCH IN TOXICOLOGY, 1996, 9 (02) :390-396

[2] INTERACTION OF NITROUS ACID WITH HYDROGEN PEROXIDE AND WITH WATER [J].

ANBAR, M ;

TAUBE, H .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1954, 76 (24) :6243-6247

[3] Direct EPR detection of the carbonate radical anion produced from peroxynitrite and carbon dioxide [J].

Bonini, MG ;

Radi, R ;

Ferrer-Sueta, G ;

Ferreira, AMD ;

Augusto, O .

JOURNAL OF BIOLOGICAL CHEMISTRY, 1999, 274 (16) :10802-10806

[4] Carbon dots for multiphoton bioimaging [J].

Cao, Li ;

Wang, Xin ;

Meziani, Mohammed J. ;

Lu, Fushen ;

Wang, Haifang ;

Luo, Pengju G. ;

Lin, Yi ;

Harruff, Barbara A. ;

Veca, L. Monica ;

Murray, Davoy ;

Xie, Su-Yuan ;

Sun, Ya-Ping .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2007, 129 (37) :11318-+

[5] Carbon Nanoparticles as Visible-Light Photocatalysts for Efficient CO2 Conversion and Beyond [J].

Cao, Li ;

Sahu, Sushant ;

Anilkumar, Parambath ;

Bunker, Christopher E. ;

Xu, Juan ;

Fernando, K. A. Shiral ;

Wang, Ping ;

Guliants, Elena A. ;

Tackett, Kenneth N., II ;

Sun, Ya-Ping .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2011, 133 (13) :4754-4757

[6] SINGLET MOLECULAR-OXYGEN PRODUCTION IN THE REACTION OF PEROXYNITRITE WITH HYDROGEN-PEROXIDE [J].

DI MASCIO, P ;

BECHARA, EJH ;

MEDEIROS, MHG ;

BRIVIBA, K ;

SIES, H .

FEBS LETTERS, 1994, 355 (03) :287-289

[7] Electrochemistry and electrogenerated chemiluminescence from silicon nanocrystal quantum dots [J].

Ding, ZF ;

Quinn, BM ;

Haram, SK ;

Pell, LE ;

Korgel, BA ;

Bard, AJ .

SCIENCE, 2002, 296 (5571) :1293-1297

[8] Polyamine-functionalized carbon quantum dots for chemical sensing [J].

Dong, Yongqiang ;

Wang, Ruixue ;

Li, Hao ;

Shao, Jingwei ;

Chi, Yuwu ;

Lin, Xiaomei ;

Chen, Guonan .

CARBON, 2012, 50 (08) :2810-2815

[9] Chemiluminescence of Pholasin caused by peroxynitrite [J].

Glebska, J ;

Koppenol, WH .

FREE RADICAL BIOLOGY AND MEDICINE, 2005, 38 (08) :1014-1022

[10] Formation of peroxynitrate from the reaction of peroxynitrite with CO2:: Evidence for carbonate radical production [J].

Goldstein, S ;

Czapski, G .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1998, 120 (14) :3458-3463

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