Isolation of single Pt atoms in a silver cluster: forming highly efficient silver-based cocatalysts for photocatalytic hydrogen evolution

被引：81

作者：

Du, Xu Lei ^{[1
]}

Wang, Xue Lu ^{[1
]}

Li, Yu Hang ^{[1
]}

Wang, Yu Lei ^{[1
]}

Zhao, Jun Jie ^{[1
]}

Fang, Li Jun ^{[1
]}

Zheng, Li Rong ^{[2
]}

Tong, Hua ^{[3
]}

Yang, Hua Gui ^{[1
]}

机构：

[1] East China Univ Sci & Technol, Sch Mat Sci & Engn, Key Lab Ultrafine Mat, Minist Educ, Shanghai 200237, Peoples R China

[2] Chinese Acad Sci, Inst High Energy Phys, Beijing Synchrotron Radiat Facil, Beijing 100049, Peoples R China

[3] East China Univ Sci & Technol, Sch Mat Sci & Engn, 130 Meilong Rd, Shanghai 200237, Peoples R China

来源：

CHEMICAL COMMUNICATIONS | 2017年 / 53卷 / 68期

基金：

中国博士后科学基金; 中国国家自然科学基金;

关键词：

CATALYTIC APPLICATION; GOLD NANOCLUSTERS; AU-25; CLUSTERS; OXIDATION; CARBON; NANOPARTICLES; ENHANCEMENT; PD;

D O I：

10.1039/c7cc04061j

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

The atomically controlled transition of nanohybrids and their effects on charge-carrier dynamics are highly desirable for fundamental studies in photocatalysis. Herein, for the first time, a method combining atomic monodispersity and single-atom alloy was used to prepare a new form of highly efficient silver-based cocatalysts (Ag-25 & Pt1Ag24) on graphitic carbon nitride, representing a novel photocatalytic system for hydrogen evolution.

引用

页码：9402 / 9405

页数：4

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