Attractive versus truncated repulsive supercooled liquids: The dynamics is encoded in the pair correlation function

被引:40
|
作者
Landes, Francois P. [1 ,2 ,3 ,4 ]
Biroli, Giulio [2 ]
Dauchot, Olivier [5 ]
Liu, Andrea J. [3 ]
Reichman, David R. [4 ]
机构
[1] Univ Paris Saclay, CNRS, INRIA, Lab Rech Informat,TAU Team, F-91405 Orsay, France
[2] Univ Paris Diderot, Sorbonne Paris Cite, Sorbonne Univ, Univ PSL,CNRS,ENS,Lab Phys, F-75005 Paris, France
[3] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA
[4] Columbia Univ, Dept Chem, 3000 Broadway, New York, NY 10027 USA
[5] PSL Res Univ, ESPCI ParisTech, CNRS, UMR Gulliver 7083, 10 Rue Vauquelin, F-75005 Paris, France
关键词
MODE-COUPLING THEORY; LENNARD-JONES MIXTURE; SIMULATIONS; FORCES;
D O I
10.1103/PhysRevE.101.010602
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
We compare glassy dynamics in two liquids that differ in the form of their interaction potentials. Both systems have the same repulsive interactions but one has also an attractive part in the potential. These two systems exhibit very different dynamics despite having nearly identical pair correlation functions. We demonstrate that a properly weighted integral of the pair correlation function, which amplifies the subtle differences between the two systems, correctly captures their dynamical differences. The weights are obtained from a standard machine learning algorithm.
引用
收藏
页数:5
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