Room temperature ferromagnetism in ZnO films due to defects

被引:321
作者
Xu, Qingyu [1 ]
Schmidt, Heidemarie [1 ]
Zhou, Shengqiang [1 ]
Potzger, Kay [1 ]
Helm, Manfred
Hochmuth, Holger [2 ]
Lorenz, Michael [2 ]
Setzer, Annette [2 ]
Esquinazi, Pablo [2 ]
Meinecke, Christoph [2 ]
Grundmann, Marius [2 ]
机构
[1] Forschungszentrum Dresden Rossendorf eV, Inst Ionenstrahlphys & Matforsch, D-01328 Dresden, Germany
[2] Univ Leipzig, Inst Expt Phys 2, D-04103 Leipzig, Germany
关键词
D O I
10.1063/1.2885730
中图分类号
O59 [应用物理学];
学科分类号
摘要
ZnO films were prepared by pulsed laser deposition on a-plane sapphire substrates under N-2 atmosphere. Ferromagnetic loops were obtained with the superconducting quantum interference device at room temperature, which indicate a Curie temperature much above room temperature. No clear ferromagnetism was observed in intentionally Cu-doped ZnO films. This excludes that Cu doping into ZnO plays a key role in tuning the ferromagnetism in ZnO. 8.8% negative magnetoresistance probed at 5 K at 60 kOe on ferromagnetic ZnO proves the lack of s-d exchange interaction. Anomalous Hall effect (AHE) was observed in ferromagnetic ZnO as well as in nonferromagnetic Cu-doped ZnO films, indicating that AHE does not uniquely prove ferromagnetism. The observed ferromagnetism in ZnO is attributed to intrinsic defects. (c) 2008 American Institute of Physics.
引用
收藏
页数:3
相关论文
共 21 条
[1]   Enhancement of ferromagnetism upon thermal annealing in pure ZnO [J].
Banerjee, S. ;
Mandal, M. ;
Gayathri, N. ;
Sardar, M. .
APPLIED PHYSICS LETTERS, 2007, 91 (18)
[2]  
BUCHHOLZ B, 2005, APPL PHYS LETT, V87
[3]   Magnetic scattering of spin polarized carriers in (In,Mn)Sb dilute magnetic semiconductor -: art. no. 227203 [J].
Csontos, M ;
Wojtowicz, T ;
Liu, X ;
Dobrowolska, M ;
Jankó, B ;
Furdyna, JK ;
Mihály, G .
PHYSICAL REVIEW LETTERS, 2005, 95 (22)
[4]   Zener model description of ferromagnetism in zinc-blende magnetic semiconductors [J].
Dietl, T ;
Ohno, H ;
Matsukura, F ;
Cibert, J ;
Ferrand, D .
SCIENCE, 2000, 287 (5455) :1019-1022
[5]   Appearance of room-temperature ferromagnetism in Cu-doped TiO2-δ films -: art. no. 161313 [J].
Duhalde, S ;
Vignolo, MF ;
Golmar, F ;
Chiliotte, C ;
Torres, CER ;
Errico, LA ;
Cabrera, AF ;
Rentería, M ;
Sánchez, FH ;
Weissmann, M .
PHYSICAL REVIEW B, 2005, 72 (16)
[6]  
Esquinazi P., 2007, HDB MAGNETISM ADV MA, V4, P2256
[7]   Magnetism of Co-doped ZnO thin films [J].
Gacic, Milan ;
Jakob, Gerhard ;
Herbort, Christian ;
Adrian, Hermann ;
Tietze, Thomas ;
Brueck, Sebastian ;
Goering, Eberhard .
PHYSICAL REVIEW B, 2007, 75 (20)
[8]   Observation of ferromagnetism at room temperature in ZnO thin films [J].
Hong, Nguyen Hoa ;
Sakai, Joe ;
Brize, Virginie .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2007, 19 (03)
[9]  
JUNGWIRTH T, 2004, PHYS REV B, V72
[10]   Ferromagnetism of ZnO and GaN:: A review [J].
Liu, C ;
Yun, F ;
Morkoç, H .
JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS, 2005, 16 (09) :555-597