Impact of emission controls on air quality in Beijing during the 2015 China Victory Day Parade: Implication from organic aerosols

被引:20
|
作者
Ren, Yanqin [1 ]
Li, Hong [1 ,2 ]
Meng, Fan [1 ]
Wang, Gehui [3 ,4 ,5 ]
Zhang, Hao [1 ]
Yang, Ting [1 ]
Li, Wenjun [1 ]
Ji, Yuanyuan [1 ]
Bi, Fang [1 ]
Wang, Xuezhong [1 ]
机构
[1] Chinese Res Inst Environm Sci, State Key Lab Environm Criteria & Risk Assessment, Beijing 100012, Peoples R China
[2] Nanjing Univ Informat Sci & Technol, Collaborat Innovat Ctr Atmospher Environm & Equip, Nanjing 210044, Jiangsu, Peoples R China
[3] East China Normal Univ, Sch Geog Sci, Minist Educ, Key Lab Geosci Informat Sci, Shanghai 200041, Peoples R China
[4] Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian 710061, Shaanxi, Peoples R China
[5] Chinese Acad Sci, Inst Urban Environm, Ctr Excellence Reg Atmospher Environm, Xiamen 361021, Peoples R China
关键词
Parade Blue; Primary organic aerosols; Organic acids; Health risk assessment; Strengthening control measures; POLYCYCLIC AROMATIC-HYDROCARBONS; DICARBOXYLIC-ACIDS; ATMOSPHERIC AEROSOLS; SOURCE APPORTIONMENT; SEASONAL-VARIATIONS; PARTICULATE MATTER; SIZE DISTRIBUTION; INLAND CHINA; WINTER HAZE; URBAN;
D O I
10.1016/j.atmosenv.2018.10.061
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
To evaluate the influence of the implementation of emission reduction measures on air quality during the 2015 China Victory Day Parade, the characteristics of organic aerosols in particulate matter with a diameter less than 2.5 gm (PM2.5) were analyzed from 11 August to 10 September 2015 in Beijing, China. The average concentration of PM2.5 decreased by 64% during the 2015 China Victory Day Parade compared with that before the event. Local emissions were the main PM2.5 sources during the 2015 China Victory Day Parade; cooking and traffic emission were two significant contributors. During the 2015 China Victory Day Parade, the average concentrations of levoglucosan and dehydroabietic acid decreased by 31% and 12%, respectively, indicating the significant effects of regional air pollution controls on air quality. 17 alpha(H), 21 beta(H)-30-Norhopane and 17 alpha(H), 21 beta(H)-hopane concentrations decreased continuously throughout the entire study period, suggesting the significant effect of the "odd-even" traffic restrictions implemented. Similarly, o-phthalic acid, succinic acid, and 2,3-dihydroxy-4-oxopentanoic acid (DPA) concentrations also significantly decreased during the Parade, with reductions of 63, 50, and 61%, respectively, compared with before the event. Photochemical oxidation played an important role in the formation of o-phthalic acid, while the formation of DPA was influenced by both photochemical oxidation and liquid-phase chemical reactions. The lung cancer risk, caused by inhalation exposure to polycyclic aromatic hydrocarbons, to the exposed populations decreased by 40% during the 2015 China Victory Day Parade, the enhanced control measures implemented during Parade Blue would also have positive influence on the human health.
引用
收藏
页码:207 / 214
页数:8
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