Formation of two-dimensional concentration pulses on microdesigned composite catalyst surfaces

被引：21
作者：
Pollmann, M
Rotermund, HH
Ertl, G
Li, XJ
Kevrekidis, IG
机构：
[1] Max Planck Gesell, Fritz Haber Inst, D-14195 Berlin, Germany
[2] Princeton Univ, Dept Chem Engn, Princeton, NJ 08544 USA
来源：
PHYSICAL REVIEW LETTERS | 2001年 / 86卷 / 26期
关键词：
D O I：
10.1103/PhysRevLett.86.6038
中图分类号：
O4 [物理学];
学科分类号：
0702 ;
摘要：
We study the effect of microdesigned composite geometries on pattern formation during the catalytic oxidation of CO on Pt-Ti, Pt-Ph, and Pt-Pd composite catalysts. In particular, we find experimentally (and rationalize through modeling) that adsorbate surface transport through the second (active) component drastically affects the shapes and interactions of concentration patterns (traveling pulses) observed on pure Pt.
引用
收藏
页码：6038 / 6041
页数：4
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