Reversible Three-State Switching of Multicolor Fluorescence Emission by Multiple Stimuli Modulated FRET Processes within Thermoresponsive Polymeric Micelles

被引：211

作者：

Li, Changhua ^{[1
]}

Zhang, Yanxi ^{[1
]}

Hu, Jinming ^{[1
]}

Cheng, Jianjun ^{[2
]}

Liu, Shiyong ^{[1
]}

机构：

[1] Univ Sci & Technol China, CAS Key Lab Soft Matter Chem, Hefei Natl Lab Phys Sci Microscale, Dept Polymer Sci & Engn, Hefei 230026, Anhui, Peoples R China

[2] Univ Illinois, Dept Mat & Engn, Urbana, IL 61801 USA

来源：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | 2010年 / 49卷 / 30期

关键词：

block copolymers; fluorescence; fluorescent probes; FRET; micelles; CONJUGATED BLOCK-COPOLYMERS; POLY N-ISOPROPYLACRYLAMIDE; RARE-EARTH IONS; ENERGY-TRANSFER; THIN-FILMS; AGGREGATION BEHAVIOR; TEMPERATURE; PHOTOLUMINESCENCE; MACROMOLECULES; NANOPARTICLES;

D O I：

10.1002/anie.201002203

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Micellar traffic lights: The title FRET system (FRET=fluorescence resonance energy transfer) consists of one type of donor dye and two types of acceptor dyes. On/off fluorescence switching of the latter two dyes can be controlled by pH changes and light, respectively. This novel type of multicolor luminescent polymeric assembly can act as a ratiometric probe for pH and temperature with tunable sensitivity. (Figure Presented). © 2010 Wiley-VCH Verlag GmbH & Co. KGaA.

引用

页码：5120 / 5124

页数：5

共 45 条

[1] Thermoresponsive PS-b-PNIPAM-b-PS Micelles: Aggregation Behavior, Segmental Dynamics, and Thermal Response [J].

Adelsberger, Joseph ;

Kulkarni, Amit ;

Jain, Abhinav ;

Wang, Weinan ;

Bivigou-Koumba, Achille M. ;

Busch, Peter ;

Pipich, Vitaliy ;

Holderer, Olaf ;

Hellweg, Thomas ;

Laschewsky, Andre ;

Mueller-Buschbaum, Peter ;

Papadakis, Christine M. .

MACROMOLECULES, 2010, 43 (05) :2490-2501

[2] Light-harvesting dendrimers [J].

Adronov, A ;

Fréchet, JMJ .

CHEMICAL COMMUNICATIONS, 2000, (18) :1701-1710

[3]

[Anonymous], 2007, ANGEW CHEM

[4]

[Anonymous], 2010, ANGEW CHE

[5]

[Anonymous], ANGEW CHEM INT ED

[6] Rhodamines NN: A Novel Class of Caged Fluorescent Dyes [J].

Belov, Vladimir N. ;

Wurm, Christian A. ;

Boyarskiy, Vadim P. ;

Jakobs, Stefan ;

Hell, Stefan W. .

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2010, 49 (20) :3520-3523

[7] Reversible fluorescence modulation through energy transfer with ABC triblock copolymer micelles as scaffolds [J].

Chen, Jian ;

Zeng, Fang ;

Wu, Shuizhu ;

Zhao, Jianqing ;

Chen, Qiming ;

Tong, Zhen .

CHEMICAL COMMUNICATIONS, 2008, (43) :5580-5582

[8] A core-shell nanoparticle approach to photoreversible fluorescence modulation of a hydrophobic dye in aqueous media [J].

Chen, Jian ;

Zeng, Fang ;

Wu, Shuizhu ;

Chen, Qiming ;

Tong, Zhen .

CHEMISTRY-A EUROPEAN JOURNAL, 2008, 14 (16) :4851-4860

[9] Living free-radical polymerization by reversible addition-fragmentation chain transfer: The RAFT process [J].

Chiefari, J ;

Chong, YK ;

Ercole, F ;

Krstina, J ;

Jeffery, J ;

Le, TPT ;

Mayadunne, RTA ;

Meijs, GF ;

Moad, CL ;

Moad, G ;

Rizzardo, E ;

Thang, SH .

MACROMOLECULES, 1998, 31 (16) :5559-5562

[10] Energy transfer in dendritic macromolecules: Molecular size effects and the role of an energy gradient [J].

Devadoss, C ;

Bharathi, P ;

Moore, JS .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1996, 118 (40) :9635-9644

← 1 2 3 4 5 →