New insights into trace element wet deposition in the Himalayas: amounts, seasonal patterns, and implications

被引:45
作者
Cong, Zhiyuan [1 ]
Kang, Shichang [1 ,2 ]
Zhang, Yulan [1 ]
Gao, Shaopeng [1 ]
Wang, Zhongyan [1 ]
Liu, Bin [1 ,3 ]
Wan, Xin [1 ,3 ]
机构
[1] Chinese Acad Sci, Inst Tibetan Plateau Res, Key Lab Tibetan Environm Changes & Land Surface P, Beijing 100101, Peoples R China
[2] Chinese Acad Sci, State Key Lab Cryospher Sci, Cold & Arid Reg Environm & Engn Res Inst, Lanzhou 730000, Peoples R China
[3] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
关键词
Himalayas; Trace elements; Wet deposition; Ice core; Long-range transport; MT. QOMOLANGMA EVEREST; ATMOSPHERIC BROWN CLOUDS; ICE-CORE; HEAVY-METALS; CHEMICAL-COMPOSITION; AEROSOL-PARTICLES; TIBETAN PLATEAU; CENTRAL-ASIA; SNOW; ANTARCTICA;
D O I
10.1007/s11356-014-3496-1
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Our research provides the first complete year-long dataset of wet deposition of trace elements in the high Himalayas based on a total of 42 wet deposition events on the northern slope of Mt. Qomolangma (Everest). Except for typical crustal elements (Al, Fe, and Mn), the concentration level of most trace elements (Sc, V, Cr, Co, Ni, Cu, Zn, As, Mo, Cd, Sn, Cs, Pb, Bi, and U) are generally comparable to those preserved in snow pits and ice cores from the nearby East Rongbuk Glacier. Cadmium was the element most affected by anthropogenic emissions. No pronounced seasonal variations are observed for most trace elements despite different transport pathways. In our study, the composition of wet precipitation reflects a regional background condition and is not clearly related to specific source regions. For the trace element record from ice cores and snow pits in the Himalayas, it could be deduced that the pronounced seasonal patterns were caused by the dry deposition of trace elements (aerosols) during their long exposure to the atmosphere after precipitation events. Our findings are of value for the understanding of the trace element deposition mechanisms in the Himalayas.
引用
收藏
页码:2735 / 2744
页数:10
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