Bulk morphology and diameter distribution of single-walled carbon nanotubes synthesized by catalytic decomposition of hydrocarbons

被引:288
作者
Cheng, HM
Li, F
Sun, X
Brown, SDM
Pimenta, MA
Marucci, A
Dresselhaus, G
Dresselhaus, MS
机构
[1] Acad Sinica, Inst Met Res, Shenyang 110015, Peoples R China
[2] MIT, Dept Phys, Cambridge, MA 02139 USA
[3] MIT, Francis Bitter Natl Magnet Lab, Cambridge, MA 02139 USA
[4] MIT, Dept Elect Engn & Comp Sci, Cambridge, MA 02139 USA
基金
中国国家自然科学基金; 美国国家科学基金会;
关键词
D O I
10.1016/S0009-2614(98)00479-5
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Long and wide ropes/ribbons of single-walled carbon nanotube (SWNT) bundles with rope diameters of 100 mu m and lengths to 3 cm were synthesized by the catalytic decomposition of hydrocarbons. These ropes/ribbons consist of roughly-aligned bundles of aligned SWNTs. The SWNT diameters, as determined from HRTEM images, are 1.69 +/- 0.34 nm, which, in combination with resonant Raman scattering measurements, indicates that our SWNTs have larger diameters than those synthesized by other techniques. The larger SWNTs are promising for gas-storage applications. The easy manipulation of the ropes offer special opportunities for their characterization and applications. (C) 1998 Published by Elsevier Science B.V. All rights reserved.
引用
收藏
页码:602 / 610
页数:9
相关论文
共 23 条
[1]   Nanometre-size tubes of carbon [J].
Ajayan, PM ;
Ebbesen, TW .
REPORTS ON PROGRESS IN PHYSICS, 1997, 60 (10) :1025-1062
[2]  
BANDOW S, 1998, IN PRESS PHYS REV LE
[3]   Single-electron transport in ropes of carbon nanotubes [J].
Bockrath, M ;
Cobden, DH ;
McEuen, PL ;
Chopra, NG ;
Zettl, A ;
Thess, A ;
Smalley, RE .
SCIENCE, 1997, 275 (5308) :1922-1925
[4]  
BROWN SDM, 1998, MRS S P BOST, V496
[5]  
CHENG HM, 1998, IN PRESS APPL PHYS L, V72
[6]   Elastic properties of single-walled carbon nanotubes in compression [J].
Cornwell, CF ;
Wille, LT .
SOLID STATE COMMUNICATIONS, 1997, 101 (08) :555-558
[7]   Storage of hydrogen in single-walled carbon nanotubes [J].
Dillon, AC ;
Jones, KM ;
Bekkedahl, TA ;
Kiang, CH ;
Bethune, DS ;
Heben, MJ .
NATURE, 1997, 386 (6623) :377-379
[8]   Nanotechnology - New tricks with nanotubes [J].
Dresselhaus, MS .
NATURE, 1998, 391 (6662) :19-20
[9]  
DRESSELHAUS MS, 1996, SCI FULLENES CARBON
[10]  
DRESSELHAUS MS, 1997, UNPUB SPECIAL LECT C