Size distribution of sea-salt emissions as a function of relative humidity

被引:79
作者
Zhang, KM
Knipping, EM
Wexler, AS [1 ]
Bhave, PV
Tonnesen, GS
机构
[1] Univ Calif Davis, Dept Mech & Aeronaut Engn, Davis, CA 95616 USA
[2] Univ Calif Davis, Dept Civil & Environm Engn, Davis, CA 95616 USA
[3] Univ Calif Davis, Dept Land Air & Water Resources, Davis, CA 95616 USA
[4] Elect Power Res Inst, Palo Alto, CA 94304 USA
[5] NOAA, Air Resources Lab, Atmospher Sci Modeling Div, Res Triangle Pk, NC 27711 USA
[6] Univ Calif Riverside, Ctr Environm Res & Technol, Riverside, CA 92521 USA
关键词
sea-salt; emission; size distribution; size correction; relative humidity; atmospheric modeling; aerosol thermodynamics;
D O I
10.1016/j.atmosenv.2005.02.032
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
This note presents a straightforward method to correct sea-salt-emission particle-size distributions according to local relative humidity. The proposed method covers a wide range of relative humidity (0.45-0.99) and its derivation incorporates recent laboratory results on sea-salt properties. The formulas are given as functions of relative humidity and compared with growth factors derived from earlier theoretical work. Application of this method to several common open-ocean and surf-zone sea-salt-particle source functions is described. The resulting sea-salt-emission aerosol distributions can be used directly in atmospheric model simulations without further correction. (c) 2005 Elsevier Ltd. All rights reserved.
引用
收藏
页码:3373 / 3379
页数:7
相关论文
共 20 条
[1]   SEA SPRAY AND THE TURBULENT AIR-SEA HEAT FLUXES [J].
ANDREAS, EL .
JOURNAL OF GEOPHYSICAL RESEARCH-OCEANS, 1992, 97 (C7) :11429-11441
[2]  
Andreas EL, 1989, 8911 CRREL
[3]  
Andrianova TV, 1998, MIKOL FITOPATOL, V32, P1
[4]   A BET model of the thermodynamics of aqueous multicomponent solutions at extreme concentration [J].
Clegg, SL ;
Simonson, JM .
JOURNAL OF CHEMICAL THERMODYNAMICS, 2001, 33 (11) :1457-1472
[5]   Production of sea spray aerosol in the surf zone [J].
de Leeuw, G ;
Neele, FP ;
Hill, M ;
Smith, MH ;
Vignali, E .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2000, 105 (D24) :29397-29409
[6]   Effect of sea salt and calcium carbonate interactions with nitric acid on the direct dry deposition of nitrogen to Tampa Bay, Florida [J].
Evans, MSC ;
Campbell, SW ;
Bhethanabotla, V ;
Poor, ND .
ATMOSPHERIC ENVIRONMENT, 2004, 38 (29) :4847-4858
[7]  
FITZGERALD JW, 1975, J APPL METEOROL, V14, P1044, DOI 10.1175/1520-0450(1975)014<1044:AFFTES>2.0.CO
[8]  
2
[9]  
Gerber H. E, 1985, RELATIVE HUMIDITY PA
[10]   Modeling sea-salt aerosols in the atmosphere .1. Model development [J].
Gong, SL ;
Barrie, LA ;
Blanchet, JP .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1997, 102 (D3) :3805-3818