Parametric four-wave mixing in the 3d and 4d Rydberg states of NO

被引:1
|
作者
Sugita, A [1 ]
Ikeda, M [1 ]
Tsukiyama, K [1 ]
机构
[1] Sci Univ Tokyo, Fac Sci, Dept Chem, Shinjuku Ku, Tokyo 1628601, Japan
来源
APPLIED PHYSICS B-LASERS AND OPTICS | 1998年 / 67卷 / 02期
关键词
D O I
10.1007/s003400050502
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
The parametric four-wave mixing (PFWM) processes via the 3d sigma, pi H(2)Sigma(+), H'(2)Pi(+/-)(nu' = 2), and 4d sigma, pi O-2 Sigma(+), O'(2)Pi(+/-) (nu' = 0) Rydberg states of NO molecules are described. The analyses of the two-photon excitation functions and infrared emission spectra revealed that only the (2)Pi-component was involved in PFWM, This is in good accordance with the absence of amplified spontaneous emission (ASE) in the (2)Sigma(+) and (2)Pi(+) components due to their predissociative character. Results provide some support for the mechanism that the generation of the vacuum ultraviolet radiation was brought by PFWM in which ASE served as a third driving wave.
引用
收藏
页码:253 / 256
页数:4
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