The Statistical Mechanics of Dynamic Pathways to Self-Assembly

被引：182

作者：

Whitelam, Stephen ^{[1
]}

Jack, Robert L. ^{[2
]}

机构：

[1] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA

[2] Univ Bath, Dept Phys, Bath BA2 7AY, Avon, England

来源：

ANNUAL REVIEW OF PHYSICAL CHEMISTRY, VOL 66 | 2015年 / 66卷

基金：

英国工程与自然科学研究理事会;

关键词：

phase change; thermodynamics; dynamics; CRYSTAL-NUCLEATION; NONCLASSICAL NUCLEATION; 2-DIMENSIONAL CRYSTALS; HOMOGENEOUS NUCLEATION; DNA; PROTEIN; CRYSTALLIZATION; GROWTH; SYMMETRY; CLUSTERS;

D O I：

10.1146/annurev-physchem-040214-121215

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

This review describes some important physical characteristics of the pathways (i.e., dynamical processes) by which molecular, nanoscale, and micrometer-scale self-assembly occurs. We highlight the existence of features of self-assembly pathways that are common to a wide range of physical systems, even though those systems may differ with respect to their microscopic details. We summarize some existing theoretical descriptions of self-assembly pathways and highlight areas-notably, the description of self-assembly pathways that occur far from equilibrium-that are likely to become increasingly important.

引用

页码：143 / 163

页数：21

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