Study of a winter PM episode in Istanbul using the high resolution WRF/CMAQ modeling system

被引:63
作者
Im, Ulas [1 ,5 ]
Markakis, Kostandinos [2 ]
Unal, Alper [3 ]
Kindap, Tayfun [3 ]
Poupkou, Anastasia [2 ]
Incecik, Selahattin [4 ]
Yenigun, Orhan [1 ]
Melas, Dimitros [2 ]
Theodosi, Christina [5 ]
Mihalopoulos, Nikos [5 ]
机构
[1] Bogazici Univ, Inst Environm Sci, TR-34342 Istanbul, Turkey
[2] Aristotle Univ Thessaloniki, Dept Phys, Lab Atmospher Phys, Thessaloniki 54124, Greece
[3] Istanbul Tech Univ, Eurasia Inst Earth Sci, TR-80626 Istanbul, Turkey
[4] Istanbul Tech Univ, Dept Meteorol, TR-80626 Istanbul, Turkey
[5] Univ Crete, Dept Chem, Environm Chem Proc Lab, Iraklion 71003, Greece
关键词
Air quality modeling; Aerosol; Chemical composition; Istanbul; WRF; CMAQ; MAJOR PHOTOCHEMICAL POLLUTANTS; AIR-QUALITY; PART I; TRANSPORT; CMAQ; PERFORMANCE; EMISSIONS; EUROPE;
D O I
10.1016/j.atmosenv.2010.05.036
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
High winter-time PM10, sulfate, nitrate and ammonium levels in Istanbul were investigated using a high resolution WRF/CMAQ mesoscale model system. A model-ready anthropogenic emission inventory on 2 km spatial resolution was developed for the area and the present study is the first attempt to test these emissions. The results suggested that the system was capable of producing the magnitudes. PM10 levels calculated by the model underestimated the observations with an average of 10 per cent at Bogazici University sampling station, whereas an overestimation of 12 per cent is calculated for all stations. High uncertainties, particularly in traffic and coal combustion, led to over estimations around emission hot spots. Base case results together with the sensitivity studies pointed significant contribution of local sources, pointing to the need of control strategies focusing on primary particulate emissions. (C) 2010 Elsevier Ltd. All rights reserved.
引用
收藏
页码:3085 / 3094
页数:10
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