Preparation and Characterization of Mesoporous TiO2 Sphere/g-C3N4 Nanosheets for Photocatalytic Behaviors

被引:8
作者
Seong, Dong Beom [1 ]
Park, Soo-Jin [1 ]
机构
[1] Inha Univ, Dept Chem, 100 Inha Ro, Incheon 402751, South Korea
基金
新加坡国家研究基金会;
关键词
Photocatalysis; Graphitic Carbon Nitride; Degradation; Rhodamine B; WATER; ANATASE; SPHERES; G-C3N4; TIO2-GRAPHENE; PERFORMANCE; FABRICATION; STRATEGY; REMOVAL; FACETS;
D O I
10.1166/jnn.2019.17056
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Composites consisting of mesoporous titanium dioxide spheres/graphitic carbon nitride (GCN-TiO2) were synthesized via a sol-gel and hydrothermal methods. The photocatalytic degradation of pollutants by the TiO2 spheres was evaluated based on the degradation of Rhodamine B (Rh B). In particular, the composites (GCN-TiO2) containing 7 wt% GCN exhibited excellent photocatalytic activity. Owing to the presence of GCN, the composites showed improved light absorption capability, pair lifetime, adsorption capacity, and a reduced band gap energy (from 3.12 to 2.65 eV). Further, the composites showed excellent durability and stability even after fifth cycles.
引用
收藏
页码:6247 / 6255
页数:9
相关论文
共 51 条
[1]  
[Anonymous], APPL CATAL B, V49, P1, DOI [10.1016/j.apcatb.2003.11.010., DOI 10.1016/J.APCATB.2003.11.010]
[2]   Controlled Fabrication of Multiwall Anatase TiO2 Nanotubular Architectures [J].
Bae, Changdeuck ;
Yoon, Youngjin ;
Yoo, Hyunjun ;
Han, Dongil ;
Cho, Jinhan ;
Lee, Byoung H. ;
Sung, Myung M. ;
Lee, MinGun ;
Kim, Jiyoung ;
Shin, Hyunjung .
CHEMISTRY OF MATERIALS, 2009, 21 (13) :2574-2576
[3]   Characterization and Photocatalytic Activity of Ag-Cu/TiO2 Nanoparticles Prepared by Sol-Gel Method [J].
Behnajady, Mohammad A. ;
Eskandarloo, Hamed .
JOURNAL OF NANOSCIENCE AND NANOTECHNOLOGY, 2013, 13 (01) :548-553
[4]   Electrochemical technologies in wastewater treatment [J].
Chen, GH .
SEPARATION AND PURIFICATION TECHNOLOGY, 2004, 38 (01) :11-41
[5]   Semiconductor-based Photocatalytic Hydrogen Generation [J].
Chen, Xiaobo ;
Shen, Shaohua ;
Guo, Liejin ;
Mao, Samuel S. .
CHEMICAL REVIEWS, 2010, 110 (11) :6503-6570
[6]   Recent developments in photocatalytic water treatment technology: A review [J].
Chong, Meng Nan ;
Jin, Bo ;
Chow, Christopher W. K. ;
Saint, Chris .
WATER RESEARCH, 2010, 44 (10) :2997-3027
[7]   Removal of heavy metal ions from wastewaters: A review [J].
Fu, Fenglian ;
Wang, Qi .
JOURNAL OF ENVIRONMENTAL MANAGEMENT, 2011, 92 (03) :407-418
[8]   One-dimensional TiO2 Nanotube Photocatalysts for Solar Water Splitting [J].
Ge, Mingzheng ;
Li, Qingsong ;
Cao, Chunyan ;
Huang, Jianying ;
Li, Shuhui ;
Zhang, Songnan ;
Chen, Zhong ;
Zhang, Keqin ;
Al-Deyab, Salem S. ;
Lai, Yuekun .
ADVANCED SCIENCE, 2017, 4 (01)
[9]   Graphitic-C3N4-hybridized TiO2 nanosheets with reactive {001} facets to enhance the UV- and visible-light photocatalytic activity [J].
Gu, Liuan ;
Wang, Jingyu ;
Zou, Zhijuan ;
Han, Xijiang .
JOURNAL OF HAZARDOUS MATERIALS, 2014, 268 :216-223
[10]  
Hirano M, 2006, J NANOSCI NANOTECHNO, V6, P762, DOI 10.1166/jnn.2006.077