Preparation of hybrid organo-inorganic catalysts based on MSM-41 mesoporous molecular sieves and their properties in synthesis of ethyl tert-butyl ether

被引：1

作者：

Vlasenko, N. V. ^{[1
]}

Kochkin, Yu. N. ^{[1
]}

Kovalenko, A. S. ^{[1
]}

机构：

[1] Natl Acad Sci Ukraine, LV Pisarzhevsky Phys Chem Inst, Kiev, Ukraine

来源：

RUSSIAN JOURNAL OF APPLIED CHEMISTRY | 2009年 / 82卷 / 12期

关键词：

LIQUID-PHASE SYNTHESIS; SITE ACCESSIBILITY; ACID; ZEOLITES; ADSORPTION; MTBE; ISOBUTENE; SILICA;

D O I：

10.1134/S1070427209120155

中图分类号：

O69 [应用化学];

学科分类号：

081704 ;

摘要：

A series of sulfoorganosilica (vinyl-containing) catalysts based on MSM-41 mesoporous molecular sieves were prepared by template synthesis. The structure and properties of these catalysts and their catalytic characteristics in synthesis of ethyl tert-butyl ether were examined.

引用

页码：2166 / 2173

页数：8

共 31 条

[1] Synthesis, characterization and catalytic activity of ZSM-5 zeolites having variable silicon-to-aluminum ratios [J].

Ali, MA ;

Brisdon, B ;

Thomas, WJ .

APPLIED CATALYSIS A-GENERAL, 2003, 252 (01) :149-162

[2] THE HYDROPHOBICITY INDEX - A NEW METHOD FOR THE CHARACTERIZATION OF SURFACE-PROPERTIES OF ZEOLITE ADSORBENTS [J].

BERKE, CH ;

KISS, A ;

KLEINSCHMIT, P ;

WEITKAMP, J .

CHEMIE INGENIEUR TECHNIK, 1991, 63 (06) :623-625

[3] Liquid phase synthesis of MTBE from methanol and isobutene over acid zeolites and amberlyst-15 [J].

Collignon, F ;

Loenders, R ;

Martens, JA ;

Jacobs, PA ;

Poncelet, G .

JOURNAL OF CATALYSIS, 1999, 182 (02) :302-312

[4] Comparative vapor phase synthesis of ETBE from ethanol and isobutene over different acid zeolites [J].

Collignon, F ;

Poncelet, G .

JOURNAL OF CATALYSIS, 2001, 202 (01) :68-77

[5] Catalysis and polymer networks -: the role of morphology and molecular accessibility [J].

Corain, B ;

Zecca, M ;

Jerábek, K .

JOURNAL OF MOLECULAR CATALYSIS A-CHEMICAL, 2001, 177 (01) :3-20

[6] Combined alkyl and sulfonic acid functionalization of MCM-41-type silica -: Part 1.: Synthesis and characterization [J].

Díaz, I ;

Márquez-Alvarez, C ;

Mohino, F ;

Pérez-Pariente, J ;

Sastre, E .

JOURNAL OF CATALYSIS, 2000, 193 (02) :283-294

[7] Etherification on zeolites: MTBE synthesis [J].

Goodwin, JG ;

Natesakhawat, S ;

Nikolopoulos, AA ;

Kim, SY .

CATALYSIS REVIEWS-SCIENCE AND ENGINEERING, 2002, 44 (02) :287-320

[8] Past, present, and future of periodic mesoporous organosilicas - The PMOs [J].

Hatton, B ;

Landskron, K ;

Whitnall, W ;

Perovic, D ;

Ozin, GA .

ACCOUNTS OF CHEMICAL RESEARCH, 2005, 38 (04) :305-312

[9] A comparative study of methyl-tert-butyl ether synthesis on zeolites HY, HBeta, HBeta/F and HZSM-5 by in situ MAS NMR spectroscopy under flow conditions and on-line gas chromatography [J].

Horvath, T ;

Seiler, M ;

Hunger, M .

APPLIED CATALYSIS A-GENERAL, 2000, 193 (1-2) :227-236

[10] MTBE - To what extent will past releases contaminate community water supply wells? [J].

Johnson, R ;

Pankow, J ;

Bender, D ;

Price, C ;

Zogorski, J .

ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2000, 34 (09) :210A-+

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