Graphene oxide as solid-state electron mediator enhanced photocatalytic activities of GO-Ag3PO4/Bi2O3 Z-scheme photocatalyst efficiently by visible-light driven

被引:16
|
作者
Wang, Jixiang [1 ]
Shen, Hongqiang [2 ]
Dai, Xiaohui [1 ]
Li, Chunmei [3 ]
Shi, Weidong [1 ]
Yan, Yongsheng [1 ]
机构
[1] Jiangsu Univ, Sch Chem & Chem Engn, Zhenjiang, Peoples R China
[2] Jiangsu Univ, Sch Mat Sci & Engn, Zhenjiang, Peoples R China
[3] Jiangsu Univ, Inst Green Chem & Chem Technol, Zhenjiang, Peoples R China
基金
中国国家自然科学基金;
关键词
Z-scheme; graphene; photocatalytic; tetracycline; Ag3PO4; HIGHLY EFFICIENT; FACILE SYNTHESIS; H-2; EVOLUTION; CO2; REDUCTION; DEGRADATION; NANOPARTICLES; PERFORMANCE; COMPOSITES; SHEETS; AG3PO4;
D O I
10.1080/10667857.2018.1455385
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The photocatalytic technology provides a simple and effective strategy for the ever-increasing environmental and energy problem. In this work, we put forward a practical method to facilitate effectively the separation of photogenerated electrons and holes by addition of graphene oxide in Ag3PO4 and Bi2O3 nanocrystals semiconductor composite. Compared with GO-single component, the three-component GO-Ag3PO4/Bi2O3 composites with the optimum Ag3PO4/Bi2O3 ratio (6:4) and content of GO (6 wt-%) presented a further improvement on the photodegradation of tetracycline by visible light irradiation driven. GO served as a medium is used to effectively transfer of the photogenerated electrons from the conduction band Bi2O3 of to the valence band of Ag3PO4, the Z-Scheme photocatalytic degradation mechanism was proposed. Our work provides an effective method for development of pragmatic photocatalyst in present environmental pollution, energy problems and other related fields.
引用
收藏
页码:421 / 432
页数:12
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