Near-resonant high order nonlinear absorption of ZnO thin films

被引:44
作者
Chan, Yun-Pei [1 ,2 ]
Lin, Ja-Hon [3 ]
Hsu, Chih-Chang [1 ,2 ]
Hsieh, Wen-Feng [1 ,2 ]
机构
[1] Natl Chiao Tung Univ, Dept Photon, Hsinchu 30050, Taiwan
[2] Natl Chiao Tung Univ, Inst Electroopt Engn, Hsinchu 30050, Taiwan
[3] Natl Taipei Univ Technol, Dept Electroopt Engn, Taipei 10608, Taiwan
来源
OPTICS EXPRESS | 2008年 / 16卷 / 24期
关键词
D O I
10.1364/OE.16.019900
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Nonlinear optical absorption of ZnO thin film grown by the laser molecular beam epitaxy was investigated by the Z-scan method using a frequency-doubled femtosecond Ti:sapphire laser. Due to near-exciton resonance, an enormous enhancement of two photon absorption (TPA) is about 3000 cm/GW at 390 nm which is about 6.5 times larger than the previously reported at two-photon exciton resonance in near-IR regime and 710 times larger than that of ZnO bulk measured at 532 nm. Besides, the free-carrier absorption resulting from linear absorption and TPA becomes essential when the excitation approaches the exciton resonance. (C) 2008 Optical Society of America
引用
收藏
页码:19900 / 19908
页数:9
相关论文
共 23 条
  • [1] NONLINEAR REFRACTIVE-INDEX OF OPTICAL-CRYSTALS
    ADAIR, R
    CHASE, LL
    PAYNE, SA
    [J]. PHYSICAL REVIEW B, 1989, 39 (05) : 3337 - 3350
  • [2] High temperature excitonic stimulated emission from ZnO epitaxial layers
    Bagnall, DM
    Chen, YF
    Zhu, Z
    Yao, T
    Shen, MY
    Goto, T
    [J]. APPLIED PHYSICS LETTERS, 1998, 73 (08) : 1038 - 1040
  • [3] Second harmonic generation in laser ablated zinc oxide thin films
    Cao, H
    Wu, JY
    Ong, HC
    Dai, JY
    Chang, RPH
    [J]. APPLIED PHYSICS LETTERS, 1998, 73 (05) : 572 - 574
  • [4] Multi-photon excitation UV emission by femtosecond pulses and nonlinearity in ZnO single crystal
    Dong, Zhi-Wei
    Zhang, Chun-Feng
    You, Guan-Jun
    Qiu, Xue-Qiong
    Liu, Kang-Jun
    Yan, Yong-Li
    Qian, Shi-Xiong
    [J]. JOURNAL OF PHYSICS-CONDENSED MATTER, 2007, 19 (21)
  • [5] Two-photon-induced excited-state absorption: Theory and experiment
    Gu, Bing
    Ji, Wei
    Patil, P. S.
    Dharmaprakash, S. M.
    Wang, Hui-Tian
    [J]. APPLIED PHYSICS LETTERS, 2008, 92 (09)
  • [6] Optical nonlinearity of ZnO microcrystallite enhanced by interfacial state
    Han, YB
    Han, JB
    Ding, S
    Chen, DJ
    Wang, QQ
    [J]. OPTICS EXPRESS, 2005, 13 (23): : 9211 - 9216
  • [7] Room-temperature ultraviolet nanowire nanolasers
    Huang, MH
    Mao, S
    Feick, H
    Yan, HQ
    Wu, YY
    Kind, H
    Weber, E
    Russo, R
    Yang, PD
    [J]. SCIENCE, 2001, 292 (5523) : 1897 - 1899
  • [8] Nonlinear optical characteristics of self-assembled films of ZnO
    Irimpan, Litty
    Deepthy, A.
    Krishnan, Bindu
    Nampoori, V. P. N.
    Radhakrishnan, P.
    [J]. APPLIED PHYSICS B-LASERS AND OPTICS, 2008, 90 (3-4): : 547 - 556
  • [9] LI CHK, 2001, OPT COMMUN, V190, P6
  • [10] Two-photon resonance assisted huge nonlinear refraction and absorption in ZnO thin films
    Lin, JH
    Chen, YJ
    Lin, HY
    Hsieh, WF
    [J]. JOURNAL OF APPLIED PHYSICS, 2005, 97 (03)