E fficient heterogeneous Fenton -like catalysis of Fe -doped SAPO-44 zeolite synthesized from bauxite and rice husk

被引:21
作者
Zhang, Qiongdan [1 ]
Wang, Qiongsheng [1 ]
Wang, Shiming [1 ]
机构
[1] Fujian Normal Univ, Coll Chem & Mat Sci, Fuzhou 350007, Peoples R China
关键词
MOLECULAR-SIEVES; METHYLENE-BLUE; FE-ZSM-5; CATALYSTS; MESOPOROUS SILICA; SINGLE-CRYSTALS; EFFICIENT; METHANOL; REMOVAL; OXIDE; DEGRADATION;
D O I
10.1016/j.cplett.2020.137598
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
In this article, the Fe-containing silicoaluminophosphate (MeSAPO-44-RH) zeolite is successfully prepared by natural bauxite and rice husk as materials in super-concentrated system. The zeolite structure improves the dispersity of Fe3+ ions, and rice husk promotes Fe incorporation of skeleton, which effectively enhance the redox activity and stability of the skeleton-Fe. MeSAPO-44-RH displays excellent Fenton-like reaction performance, which achieves degrade reactive bright red (X-3B) nearly 100% within 60 min. Meanwhile, it exhibits superior cyclic stability without deactivation for 10 runs experiment. Our strategy provides a clean, green and efficient process route for bauxite and biomass waste. © 2020 Elsevier B.V.
引用
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页数:9
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