Quantification of seasonal sediment and phosphorus transport dynamics in an agricultural watershed using radiometric fingerprinting techniques

被引:42
作者
Huisman, Natalie L. H. [1 ]
Karthikeyan, K. G. [2 ]
Lamba, Jasmeet [2 ]
Thompson, Anita M. [2 ]
Peaslee, Graham [3 ]
机构
[1] Union Coll, Dept Chem, Schenectady, NY 12308 USA
[2] Univ Wisconsin, Dept Biol Syst Engn, Madison, WI 53706 USA
[3] Hope Coll, Dept Chem, Holland, MI 49422 USA
基金
美国国家科学基金会;
关键词
Fallout radionuclides; Phosphorus; Sediment fingerprinting; Sediment sources; FLUVIAL SUSPENDED SEDIMENT; SOURCE POLLUTION MODEL; FALLOUT RADIONUCLIDES; MANAGEMENT TOOL; RIVER-BASINS; STREAM-FLOW; CATCHMENT; AGGREGATION; BERYLLIUM-7; WISCONSIN;
D O I
10.1007/s11368-013-0769-0
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Phosphorus (P) is a limiting nutrient for most US Midwestern aquatic systems and, therefore, increases of P, through point or non-point sources (NPS) of pollution such as agriculture, causes eutrophication. Identifying specific NPS contributions (e.g., upland vs. stream channels) for sediments and P is difficult due to the distributed nature of the pollution. Therefore, studies which link the spatial and temporal aspects of sediment and P transport in these systems can help better characterize the extent of NPS pollution. Our study used fingerprinting techniques to determine sources of sediments in an agricultural watershed (the North Fork of the Pheasant Branch watershed; 12.4 km(2) area) in Wisconsin, USA, during the spring, summer, and fall seasons of 2009. The primary sources considered were uplands (cultivated fields), stream bank, and streambed. The model used fallout radionuclides, Cs-137, and Pb-210(xs), along with total P to determine primary sediment sources. A shorter-lived fallout radioisotope, Be-7, was used to determine the sediment age and percent new sediments in streambed and suspended sediment samples (via the Be-7/Pb-210(xs) ratio). Upland areas were the primary source of suspended sediments in the stream channels followed by stream banks. The sediment age and percent new sediment for the streambed and suspended sediments showed that the channel contained and transported newer (or more recently tagged with Be-7) sediments in the spring season (9-131 days sediment age), while relatively old sediments (165-318 days) were moving through the channel system during the fall season. Upland areas are the major contributors to in-stream suspended sediments in this watershed. Sediment resuspension in stream channels could play an important role during the later part of the year. Best management practices should be targeted in the upland areas to reduce the export of sediments and sediment-bound P from agricultural watersheds.
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页码:1724 / 1734
页数:11
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