Phosphorus removal from aqueous solutions using a synthesized adsorbent prepared from mineralized refuse and sewage sludge

被引:23
作者
Chen, Kaining [1 ]
Zhao, Keqiang [2 ]
Zhang, Houhu [2 ]
Sun, Qinfang [2 ]
Wu, Zhilin [2 ]
Zhou, Yongmin [3 ]
Zhong, Yongchao [3 ]
Ke, Fan [1 ]
机构
[1] Chinese Acad Sci, Nanjing Inst Geog & Limnol, State Key Lab Lake Sci & Environm, Nanjing, Jiangsu, Peoples R China
[2] Nanjing Inst Environm Sci, Nanjing, Jiangsu, Peoples R China
[3] Nanjing Univ Technol, Coll Mat Sci & Engn, Nanjing, Jiangsu, Peoples R China
关键词
synthesized adsorbent; mineralized refuse; sewage sludge; isotherm equations; desorbability; WASTE-WATER TREATMENT; PHOSPHATE ADSORPTION; WETLAND; RETENTION; SAND; SLAG;
D O I
10.1080/09593330.2012.758659
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Mineralized refuse and sewage sludge generated from solid waste from municipal landfills and sewage treatment plants were sintered as a cost-effective adsorbent for the removal of phosphorus. Compared with the Freundlich model, phosphorus adsorption on the synthesized adsorbent, zeolite and ironstone was best described by the Langmuir model. Based on the Langmuir model, the maximum adsorption capacity of the synthesized adsorbent (9718mgkg(-1)) was 13.7 and 25.4 times greater than those of zeolite and ironstone, respectively. The desorbability of phosphorus from the synthesized adsorbent was significantly lower than that of zeolite. Moreover, phosphorus removal using the synthesized adsorbent was more tolerant to pH fluctuations than zeolite and ironstone for the removal of phosphorus from aqueous solutions. The immobilization of phosphorus onto the synthesized adsorbent was attributed to the formation of insoluble calcium, aluminium and iron phosphorus. The heavy metal ion concentrations of the leachate of the synthesized adsorbent were negligible. The synthesized adsorbent prepared from mineralized refuse and sewage sludge was cost-effective and possessed a high adsorptive capacity for phosphorus removal from aqueous solutions.
引用
收藏
页码:1489 / 1496
页数:8
相关论文
共 36 条
[1]   Adsorption and desorption of phosphate and nitrate ions using quaternary (polypropylene-g-N,N-dimethylamino ethylmethacrylate) graft copolymer [J].
Abou Taleb, Manal F. ;
Mahmoud, Ghada A. ;
Elsigeny, Samia M. ;
Hegazy, El-Sayed A. .
JOURNAL OF HAZARDOUS MATERIALS, 2008, 159 (2-3) :372-379
[2]  
[Anonymous], 1998, STANDARD METHODS EXA, P20, DOI 10.2105/SMWW.2882.218
[3]   Reuse of dewatered aluminium-coagulated water treatment residual to immobilize phosphorus: Batch and column trials using a condensed phosphate [J].
Babatunde, A. O. ;
Zhao, Y. Q. ;
Yang, Y. ;
Kearney, P. .
CHEMICAL ENGINEERING JOURNAL, 2008, 136 (2-3) :108-115
[4]   Phosphorus removal from wastewater by mineral apatite [J].
Bellier, Nathalie ;
Chazarenc, Florent ;
Comeau, Yves .
WATER RESEARCH, 2006, 40 (15) :2965-2971
[5]  
Cao F. Y., 2009, ENV SCI MANAGE, V34, P50
[6]   Physico-chemical screening of phosphate-removing substrates for use in constructed wetland systems [J].
Drizo, A ;
Frost, CA ;
Grace, J ;
Smith, KA .
WATER RESEARCH, 1999, 33 (17) :3595-3602
[7]   Phosphorus removal by electric arc furnace steel slag and serpentinite [J].
Drizo, Aleksandra ;
Forget, Christiane ;
Chapuis, Robert P. ;
Comeau, Yves .
WATER RESEARCH, 2006, 40 (08) :1547-1554
[8]   Phosphorus retention and sorption by constructed wetland soils in Southeast Ireland [J].
Dunne, EJ ;
Culleton, N ;
O'Donovan, G ;
Harrington, R ;
Daly, K .
WATER RESEARCH, 2005, 39 (18) :4355-4362
[9]   Preparation of a new sorbent with hydrated lime and blast furnace slag for phosphorus removal from aqueous solution [J].
Gong, Guozhuo ;
Ye, Shufeng ;
Tian, Yajun ;
Wang, Qi ;
Ni, Jiandi ;
Chen, Yunfa .
JOURNAL OF HAZARDOUS MATERIALS, 2009, 166 (2-3) :714-719
[10]   Phosphate immobilization using an acidic type F fly ash [J].
Grubb, DG ;
Guimaraes, MS ;
Valencia, R .
JOURNAL OF HAZARDOUS MATERIALS, 2000, 76 (2-3) :217-236