Uniaxial strain induced band splitting in semiconducting SrTiO3

被引:16
作者
Chang, Young Jun [1 ,2 ,3 ]
Khalsa, Guru [4 ]
Moreschini, Luca [1 ]
Walter, Andrew L. [1 ,2 ]
Bostwick, Aaron [1 ]
Horn, Karsten [2 ]
MacDonald, A. H. [4 ]
Rotenberg, Eli [1 ]
机构
[1] EO Lawrence Berkeley Natl Lab, ALS, Berkeley, CA 94720 USA
[2] Max Planck Gesell, Fritz Haber Inst, Dept Phys Chem, D-14195 Berlin, Germany
[3] Univ Seoul, Dept Phys, Seoul 130743, South Korea
[4] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA
基金
瑞士国家科学基金会; 美国国家科学基金会; 新加坡国家研究基金会;
关键词
2-DIMENSIONAL ELECTRON-GAS; INTERFACES;
D O I
10.1103/PhysRevB.87.115212
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We use angle-resolved photoemission spectroscopy to study the influence of mechanically induced uniaxial strain on the electronic structure of the oxide semiconductor SrTiO3. We observe an orbital splitting between the Ti 3d(yz) and 3d(xy) bands, which are degenerate when unperturbed. Using the k center dot p method, we qualitatively explain the direction and the size of the observed energy splitting. Our comprehensive understanding of band splitting explains the strain induced mobility enhancement of electron-doped SrTiO3(3) in terms of band degeneracy breaking and reduced interband scattering. Our approach can be extended to differently strained oxide systems. DOI: 10.1103/PhysRevB.87.115212
引用
收藏
页数:5
相关论文
共 27 条
[1]   Strain and high temperature superconductivity: Unexpected results from direct electronic structure measurements in thin films [J].
Abrecht, M ;
Ariosa, D ;
Cloetta, D ;
Mitrovic, S ;
Onellion, M ;
Xi, XX ;
Margaritondo, G ;
Pavuna, D .
PHYSICAL REVIEW LETTERS, 2003, 91 (05)
[2]   Electronic phase separation at the LaAlO3/SrTiO3 interface [J].
Ariando ;
Wang, X. ;
Baskaran, G. ;
Liu, Z. Q. ;
Huijben, J. ;
Yi, J. B. ;
Annadi, A. ;
Barman, A. Roy ;
Rusydi, A. ;
Dhar, S. ;
Feng, Y. P. ;
Ding, J. ;
Hilgenkamp, H. ;
Venkatesan, T. .
NATURE COMMUNICATIONS, 2011, 2
[3]   Photo-electrochemical hydrogen generation from water using solar energy. Materials-related aspects [J].
Bak, T ;
Nowotny, J ;
Rekas, M ;
Sorrell, CC .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2002, 27 (10) :991-1022
[4]   Tailoring a two-dimensional electron gas at the LaAlO3/SrTiO3 (001) interface by epitaxial strain [J].
Bark, C. W. ;
Felker, D. A. ;
Wang, Y. ;
Zhang, Y. ;
Jang, H. W. ;
Folkman, C. M. ;
Park, J. W. ;
Baek, S. H. ;
Zhou, H. ;
Fong, D. D. ;
Pan, X. Q. ;
Tsymbal, E. Y. ;
Rzchowski, M. S. ;
Eom, C. B. .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2011, 108 (12) :4720-4724
[5]   ELASTIC CONSTANTS OF STRONTIUM TITANATE [J].
BELL, RO ;
RUPPRECHT, G .
PHYSICAL REVIEW, 1963, 129 (01) :90-&
[6]   Band Gap and Edge Engineering via Ferroic Distortion and Anisotropic Strain: The Case of SrTiO3 [J].
Berger, Robert F. ;
Fennie, Craig J. ;
Neaton, Jeffrey B. .
PHYSICAL REVIEW LETTERS, 2011, 107 (14)
[7]   2-BAND SUPERCONDUCTIVITY IN NB-DOPED SRTIO3 [J].
BINNIG, G ;
BARATOFF, A ;
HOENIG, HE ;
BEDNORZ, JG .
PHYSICAL REVIEW LETTERS, 1980, 45 (16) :1352-1355
[8]  
Bir G. L., 1974, SYMMETRY STRAIN EFFE
[9]   Electronic structure of doped d0 perovskite semiconductors [J].
Bistritzer, R. ;
Khalsa, G. ;
MacDonald, A. H. .
PHYSICAL REVIEW B, 2011, 83 (11)
[10]   Structure and correlation effects in semiconducting SrTiO3 [J].
Chang, Young Jun ;
Bostwick, Aaron ;
Kim, Yong Su ;
Horn, Karsten ;
Rotenberg, Eli .
PHYSICAL REVIEW B, 2010, 81 (23)