Label-free second harmonic and hyper Rayleigh scattering with high efficiency

被引:52
作者
Gomopoulos, Nikolaos [1 ]
Luetgebaucks, Cornelis [1 ]
Sun, Qinchao [1 ]
Macias-Romero, Carlos [1 ]
Roke, Sylvie [1 ]
机构
[1] Ecole Polytech Fed Lausanne, Sch Engn STI, Inst Bioengn IBI, Lab Fundamental BioPhoton LBP, CH-1015 Lausanne, Switzerland
基金
瑞士国家科学基金会; 欧洲研究理事会;
关键词
NONLINEAR-OPTICAL PROBE; LIGHT-SCATTERING; PARTICLE-SIZE; SURFACE; GENERATION; SPECTROSCOPY; ADSORPTION; INTERFACE; POLARIZATION;
D O I
10.1364/OE.21.000815
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We present a method to perform hyper Rayleigh scattering from aqueous solutions and second harmonic scattering measurements from unlabeled interfaces of liposomes and nanoparticles in dilute solutions. The water and interfacial response can be measured on a millisecond timescale, thus opening up the possibility to measure label-free time dependent transport processes in biological (membrane) systems. (C) 2013 Optical Society of America
引用
收藏
页码:815 / 821
页数:7
相关论文
共 40 条
[1]  
[Anonymous], 2008, HDB BIOMEDICAL NONLI
[2]   DOUBLE-QUANTUM LIGHT SCATTERING BY MOLECULES [J].
BERSOHN, R ;
PAO, YH ;
FRISCH, HL .
JOURNAL OF CHEMICAL PHYSICS, 1966, 45 (09) :3184-&
[3]   Sensing with Multipolar Second Harmonic Generation from Spherical Metallic Nanoparticles [J].
Butet, Jeremy ;
Russier-Antoine, Isabelle ;
Jonin, Christian ;
Lascoux, Noelle ;
Benichou, Emmanuel ;
Brevet, Pierre-Francois .
NANO LETTERS, 2012, 12 (03) :1697-1701
[4]   Amyloidogenic Protein Membrane Interactions: Mechanistic Insight from Model Systems [J].
Butterfield, Sara M. ;
Lashuel, Hilal A. .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2010, 49 (33) :5628-5654
[5]  
Clays K., 2008, Linear and Nonlinear Optics of Organic Materials Viii, V7049
[6]   Theory of optical second-harmonic generation from a sphere of centrosymmetric material: small-particle limit [J].
Dadap, JI ;
Shan, J ;
Heinz, TF .
JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 2004, 21 (07) :1328-1347
[7]   Analysis of second-harmonic generation by unamplified, high-repetition-rate, ultrashort laser pulses at Si(001) interfaces [J].
Dadap, JI ;
Hu, XF ;
Russell, NM ;
Ekerdt, JG ;
Lowell, JK ;
Downer, MC .
IEEE JOURNAL OF SELECTED TOPICS IN QUANTUM ELECTRONICS, 1995, 1 (04) :1145-1155
[8]   Theory of optical second-harmonic and sum-frequency scattering from arbitrarily shaped particles [J].
de Beer, Alex G. F. ;
Roke, Sylvie ;
Dadap, Jerry I. .
JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 2011, 28 (06) :1374-1384
[9]   Adsorption of a cationic dye molecule on polystyrene microspheres in colloids: Effect of surface charge and composition probed by second harmonic generation [J].
Eckenrode, HM ;
Jen, SH ;
Han, J ;
Yeh, AG ;
Dai, HL .
JOURNAL OF PHYSICAL CHEMISTRY B, 2005, 109 (10) :4646-4653
[10]   Nonlinear optical probe of biopolymer adsorption on colloidal particle surface: Poly-L-lysine on polystyrene sulfate microspheres [J].
Eckenrode, HM ;
Dai, HL .
LANGMUIR, 2004, 20 (21) :9202-9209