Numerical investigation of PEM electrolysis cell with the new interdigitated-jet hole flow field

被引:36
作者
Chen, Zhichao [1 ]
Wang, Xueye [2 ]
Liu, Cong [1 ]
Gu, Lingli [1 ]
Yin, Likun [1 ]
Xu, Chao [2 ]
Liao, Zhirong [2 ]
Wang, Zhiming [3 ]
机构
[1] China Three Gorges Corp, Sci & Technol Res Inst, Beijing 100038, Peoples R China
[2] North China Elect Power Univ, Sch Energy Power & Mech Engn, Key Lab Power Stn Energy Transfer Convers & Syst M, Beijing 102206, Peoples R China
[3] Tianjin Univ Commerce, Tianjin Key Lab Refrigerat Technol, Tianjin 300134, Peoples R China
基金
中国国家自然科学基金;
关键词
Proton exchange membrane; electrolysis cell; Interdigitated-jet hole flow field; Application mode; Structure optimization; POROUS TRANSPORT LAYER; MEMBRANE FUEL-CELL; GAS-LIQUID FLOW; WATER ELECTROLYSIS; CURRENT-DENSITY; HIGH-PRESSURE; PERFORMANCE ASSESSMENT; 2-PHASE TRANSPORT; SIMULATION; MODEL;
D O I
10.1016/j.ijhydene.2022.07.229
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The flow field structure has important influences on the mass and heat transfer and the distribution uniformity in the proton exchange membrane electrolysis cell (PEMEC). In this paper, the application and operation modes and the structural parameters of the new interdigitated-jet hole flow field (JHFF) are explored, to guide the processing of the JHFF and provide references for experimental testing. A three-dimensional and two-phase model is established to simulate the effect of JHFF on the performance of PEMEC. The results demonstrate that compared with the application of JHFF only on the anode side, the application of JHFF on both sides of the anode and cathode can increase the temperature distribution uniformity and polarization performance by 41.78% and 16.25%, respectively. By increasing the number of inlet flow channels and using the counter-flow water supply mode, the temperature distribution can be more uniform. The lower the height of jet holes, the better the normal mass transfer and polarization performance, while the worse the temperature distribution uniformity. Reducing the diameter of the inlet jet holes can improve the normal mass transfer performance in the porous electrode. Synthetically, the hole height of 0.2 mm and the hole diameter of 0.4 mm are recommended. The findings provide theoretical guidance for the practical application of JHFF in PEMEC so that the positive role of JHFF in improving electrolysis performance can be fully realized.(c) 2022 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:33177 / 33194
页数:18
相关论文
共 49 条
  • [1] Modelling and simulation of a proton exchange membrane (PEM) electrolyser cell
    Abdin, Z.
    Webb, C. J.
    Gray, E. MacA
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2015, 40 (39) : 13243 - 13257
  • [2] Performance assessment of gas crossover phenomenon and water transport mechanism in high pressure PEM electrolyzer
    Afshari, E.
    Khodabakhsh, S.
    Jahantigh, N.
    Toghyani, S.
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2021, 46 (19) : 11029 - 11040
  • [3] Analyses of heat and water transport interactions in a proton exchange membrane fuel cell
    Afshari, E.
    Jazayeri, S. A.
    [J]. JOURNAL OF POWER SOURCES, 2009, 194 (01) : 423 - 432
  • [4] Two-dimensional model of low-pressure PEM electrolyser: Two-phase flow regime, electrochemical modelling and experimental validation
    Aubras, F.
    Deseure, J.
    Kadjo, J. J. A.
    Dedigama, I.
    Majasan, J.
    Grondin-Perez, B.
    Chabriat, J. -P.
    Brett, D. J. L.
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2017, 42 (42) : 26203 - 26216
  • [5] Hydrogen: A brief overview on its sources, production and environmental impact
    Baykara, Sema Z.
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2018, 43 (23) : 10605 - 10614
  • [6] A review on PEM electrolyzer modelling: Guidelines for beginners
    Falcao, D. S.
    Pinto, A. M. F. R.
    [J]. JOURNAL OF CLEANER PRODUCTION, 2020, 261
  • [7] Measuring and modeling mass transport losses in proton exchange membrane water electrolyzers using electrochemical impedance spectroscopy
    Garcia-Navarro, J. C.
    Schulze, M.
    Friedrich, K. A.
    [J]. JOURNAL OF POWER SOURCES, 2019, 431 : 189 - 204
  • [8] Capabilities and Limitations of 3D-CFD Simulation of Anode Flow Fields of High-Pressure PEM Water Electrolysis
    Haas, Christoph
    Macherhammer, Marie-Gabrielle
    Klopcic, Nejc
    Trattner, Alexander
    [J]. PROCESSES, 2021, 9 (06)
  • [9] Modeling of two-phase transport in proton exchange membrane electrolyzer cells for hydrogen energy
    Han, Bo
    Mo, Jingke
    Kang, Zhenye
    Yang, Gaoqiang
    Barnhill, William
    Zhang, Feng-Yuan
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2017, 42 (07) : 4478 - 4489
  • [10] Effects of membrane electrode assembly properties on two-phase transport and performance in proton exchange membrane electrolyzer cells
    Han, Bo
    Mo, Jingke
    Kang, Zhenye
    Zhang, Feng-Yuan
    [J]. ELECTROCHIMICA ACTA, 2016, 188 : 317 - 326