Metal Oxide/Carbide/Carbon Nanocomposites: In Situ Synthesis, Characterization, Calculation, and their Application as an Efficient Counter Electrode Catalyst for Dye-Sensitized Solar Cells

被引：158

作者：

Yun, Sining ^{[1
]}

Zhang, Hong ^{[2
]}

Pu, Huihai ^{[3
]}

Chen, Junhong ^{[3
]}

Hagfeldt, Anders ^{[4
]}

Ma, Tingli ^{[2
]}

机构：

[1] Xian Univ Architecture & Technol, Sch Mat & Mineral Resources, Xian 710055, Shaanxi, Peoples R China

[2] Dalian Univ Technol, State Key Lab Fine Chem, Dalian 116024, Peoples R China

[3] Univ Wisconsin, Dept Mech Engn, Milwaukee, WI 53211 USA

[4] Uppsala Univ, Dept Phys & Analyt Chem, SE-75105 Uppsala, Sweden

来源：

ADVANCED ENERGY MATERIALS | 2013年 / 3卷 / 11期

关键词：

HIGH-PERFORMANCE; MESOPOROUS CARBON; TITANIUM NITRIDE; PLATINUM; GRAPHENE; TIO2; NANOTUBES; CARBIDES; CATHODE; DIOXIDE;

D O I：

10.1002/aenm.201300242

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

TaO- and TaC-based nanocomposites as novel and low-cost counter electrodes (CEs) in dye-sensitized solar cells (DSCs) show outstanding electrocatalytic activity and photovoltaic performance, superior to the Pt electrode. Based on the first-principles density functional theory (DFT) calculations, I3 is chemisorbed onto the TaO surface as opposed to physical adsorption on the TaC surface. The TaO-based composite is more efficient than the TaC-based composite as a CE in DSCs. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

引用

页码：1407 / 1412

页数：6

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