Host model uncertainties in aerosol radiative forcing estimates: results from the AeroCom Prescribed intercomparison study

被引:117
|
作者
Stier, P. [1 ]
Schutgens, N. A. J. [1 ]
Bellouin, N. [2 ]
Bian, H. [3 ,4 ]
Boucher, O. [5 ]
Chin, M. [4 ]
Ghan, S. [6 ]
Huneeus, N. [5 ]
Kinne, S. [7 ]
Lin, G. [8 ]
Ma, X. [9 ]
Myhre, G. [10 ]
Penner, J. E. [8 ]
Randles, C. A. [4 ,11 ]
Samset, B. [10 ]
Schulz, M. [12 ]
Takemura, T. [13 ]
Yu, F. [9 ]
Yu, H. [4 ,14 ]
Zhou, C. [8 ]
机构
[1] Univ Oxford, Dept Phys, Oxford OX1 3PU, England
[2] Met Off, Hadley Ctr, Exeter, Devon, England
[3] Univ Maryland Baltimore Cty, Joint Ctr Earth Syst Technol, Baltimore, MD 21228 USA
[4] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA
[5] UPMC, CNRS, IPSL, Lab Meteorol Dynam, Paris, France
[6] Pacific NW Natl Lab, Richland, WA 99352 USA
[7] Max Planck Inst Meteorol, D-20146 Hamburg, Germany
[8] Univ Michigan, Dept Atmospher Ocean & Space Sci, Ann Arbor, MI 48109 USA
[9] SUNY Albany, Atmospher Sci Res Ctr, Albany, NY 12222 USA
[10] CICERO, Oslo, Norway
[11] Morgan State Univ, GESTAR, Baltimore, MD 21239 USA
[12] Norwegian Meteorol Inst, Oslo, Norway
[13] Kyushu Univ, Appl Mech Res Inst, Fukuoka 8168580, Japan
[14] Univ Maryland, Earth Syst Sci Interdisciplinary Ctr, College Pk, MD 20742 USA
基金
美国国家科学基金会; 英国自然环境研究理事会; 美国国家航空航天局;
关键词
SATELLITE; SIMULATION; SENSITIVITY; SULFATE; ALBEDO; CODE;
D O I
10.5194/acp-13-3245-2013
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Simulated multi-model "diversity" in aerosol direct radiative forcing estimates is often perceived as a measure of aerosol uncertainty. However, current models used for aerosol radiative forcing calculations vary considerably in model components relevant for forcing calculations and the associated "host-model uncertainties" are generally convoluted with the actual aerosol uncertainty. In this AeroCom Prescribed intercomparison study we systematically isolate and quantify host model uncertainties on aerosol forcing experiments through prescription of identical aerosol radiative properties in twelve participating models. Even with prescribed aerosol radiative properties, simulated clear-sky and all-sky aerosol radiative forcings show significant diversity. For a purely scattering case with globally constant optical depth of 0.2, the global-mean all-sky top-of-atmosphere radiative forcing is -4.47 Wm(-2) and the inter-model standard deviation is 0.55 Wm(-2), corresponding to a relative standard deviation of 12 %. For a case with partially absorbing aerosol with an aerosol optical depth of 0.2 and single scattering albedo of 0.8, the forcing changes to 1.04 Wm(-2), and the standard deviation increases to 1.01 W-2, corresponding to a significant relative standard deviation of 97 %. However, the top-of-atmosphere forcing variability owing to absorption (subtracting the scattering case from the case with scattering and absorption) is low, with absolute (relative) standard deviations of 0.45 Wm(-2) (8 %) clear-sky and 0.62 Wm(-2) (11 %) all-sky. Scaling the forcing standard deviation for a purely scattering case to match the sulfate radiative forcing in the AeroCom Direct Effect experiment demonstrates that host model uncertainties could explain about 36% of the overall sulfate forcing diversity of 0.11 Wm(-2) in the AeroCom Direct Radiative Effect experiment. Host model errors in aerosol radiative forcing are largest in regions of uncertain host model components, such as stratocumulus cloud decks or areas with poorly constrained surface albedos, such as sea ice. Our results demonstrate that host model uncertainties are an important component of aerosol forcing uncertainty that require further attention.
引用
收藏
页码:3245 / 3270
页数:26
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