Biomimetic Durable Multifunctional Self-Cleaning Nanofibrous Membrane with Outstanding Oil/Water Separation, Photodegradation of Organic Contaminants, and Antibacterial Performances

被引：234

作者：

Ma, Wenjing ^{[1
]}

Li, Yuansheng ^{[2
]}

Zhang, Mengjie ^{[2
]}

Gao, Shuting ^{[2
]}

Cui, Jiaxin ^{[2
]}

Huang, Chaobo ^{[2
]}

Fu, Guodong ^{[1
]}

机构：

[1] Southeast Univ SEU, Coll Chem & Chem Engn, Nanjing 211189, Jiangsu, Peoples R China

[2] Nanjing Forestry Univ NFU, Jiangsu Key Lab Biomass Based Green Fuels & Chem, Coll Chem Engn, Jiangsu Prov Key Lab Chem & Utilizat Agroforest B, Nanjing 210037, Jiangsu, Peoples R China

来源：

ACS APPLIED MATERIALS & INTERFACES | 2020年 / 12卷 / 31期

基金：

中国国家自然科学基金;

关键词：

durable; zeolitic imidazolate framework-8@thiolated graphene; nanofibrous membrane; self-cleaning; oil/water separation; photodegradation of organic contaminants; antibacterial; REDUCED GRAPHENE OXIDE; OIL; SURFACES; MECHANISMS; SPONGES;

D O I：

10.1021/acsami.0c09059

中图分类号：

TB3 [工程材料学];

学科分类号：

0805 ; 080502 ;

摘要：

Wastewater pollution has always been one of the most severe worldwide environmental problems. In addition, in light of the frequent oil spills that have occurred in recent years, the treatment of oily wastewater is particularly important. In this work, a novel zeolitic imidazolate framework-8@thiolated graphene (ZIF-8@GSH) composites-based polyimide (PI) nanofibrous membrane was developed via a facile electrospinning and in situ hydrothermal synthesis approaches for effective purification of oily wastewater. The membrane showed superhydrophobicity/superoleophilicity and high separation efficiency (>99.9%) for a wide range of oil/water mixtures and water-in-oil emulsions. Besides, the membrane demonstrated excellent photocatalytic dye degradation, antibacterial, self-cleaning, and mechanochemical durable abilities, showing high potential in oily wastewater treatment and water remediation.

引用

页码：34999 / 35010

页数：12

共 63 条

[41] MOF thin films: existing and future applications [J].

Shekhah, O. ;

Liu, J. ;

Fischer, R. A. ;

Woell, Ch. .

CHEMICAL SOCIETY REVIEWS, 2011, 40 (02) :1081-1106

[42] Ultrafast Separation of Emulsified Oil/Water Mixtures by Ultrathin Free-Standing Single-Walled Carbon Nanotube Network Films [J].

Shi, Zhun ;

Zhang, Wenbin ;

Zhang, Feng ;

Liu, Xia ;

Wang, Dong ;

Jin, Jian ;

Jiang, Lei .

ADVANCED MATERIALS, 2013, 25 (17) :2422-2427

[43] Zeolitic imidazolate framework (ZIF-8) based polymer nanocomposite membranes for gas separation [J].

Song, Qilei ;

Nataraj, S. K. ;

Roussenova, Mina V. ;

Tan, Jin Chong ;

Hughes, David J. ;

Li, Wei ;

Bourgoin, Pierre ;

Alam, M. Ashraf ;

Cheetham, Anthony K. ;

Al-Muhtaseb, Shaheen A. ;

Sivaniah, Easan .

ENERGY & ENVIRONMENTAL SCIENCE, 2012, 5 (08) :8359-8369

[44] Graphene-based composite materials [J].

Stankovich, Sasha ;

Dikin, Dmitriy A. ;

Dommett, Geoffrey H. B. ;

Kohlhaas, Kevin M. ;

Zimney, Eric J. ;

Stach, Eric A. ;

Piner, Richard D. ;

Nguyen, SonBinh T. ;

Ruoff, Rodney S. .

NATURE, 2006, 442 (7100) :282-286

[45] MECHANISMS OF ACTION OF THE ANTI-MYCOTIC IMIDAZOLES [J].

SUD, IJ ;

FEINGOLD, DS .

JOURNAL OF INVESTIGATIVE DERMATOLOGY, 1981, 76 (06) :438-441

[46] Tunable Electrical Conductivity in Metal-Organic Framework Thin-Film Devices [J].

Talin, A. Alec ;

Centrone, Andrea ;

Ford, Alexandra C. ;

Foster, Michael E. ;

Stavila, Vitalie ;

Haney, Paul ;

Kinney, R. Adam ;

Szalai, Veronika ;

El Gabaly, Farid ;

Yoon, Heayoung P. ;

Leonard, Francois ;

Allendorf, Mark D. .

SCIENCE, 2014, 343 (6166) :66-69

[47] One-dimensional core-shell Zn0.1Cd0.9S/Snln4S8 heterojunction for enhanced visible light photocatalytic degradation [J].

Tang, Yunxiang ;

Zhang, Xin ;

Ma, Yuxue ;

Wang, Xiaotong ;

Su, Changhua ;

Zhang, Dafeng ;

Pu, Xipeng ;

Geng, Yanling .

SEPARATION AND PURIFICATION TECHNOLOGY, 2020, 230

[48] An Intelligent Superwetting PVDF Membrane Showing Switchable Transport Performance for Oil/Water Separation [J].

Tao, Mimi ;

Xue, Lixin ;

Liu, Fu ;

Jiang, Lei .

ADVANCED MATERIALS, 2014, 26 (18) :2943-2948

[49] ZnO-pHEMA Nanocomposites: An Ecofriendly and Reusable Material for Water Remediation [J].

Ussia, Martina ;

Di Mauro, Alessandro ;

Mecca, Tommaso ;

Cunsolo, Francesca ;

Nicotra, Giuseppe ;

Spinella, Corrado ;

Cerruti, Pierfrancesco ;

Impellizzeri, Giuliana ;

Privitera, Vittorio ;

Carroccio, Sabrina C. .

ACS APPLIED MATERIALS & INTERFACES, 2018, 10 (46) :40100-40110

[50]

Wang CC, 2014, ENERG ENVIRON SCI, V7, P2831, DOI [10.1039/c4ee01299b, 10.1039/C4EE01299B]

← 1 2 3 4 5 6 7 →