Low-Temperature Selective Catalytic Reduction of NO on an Iron Ore Catalyst in a Magnetically Fluidized Bed

被引:16
|
作者
Gui, Keting [1 ]
Liang, Hui [1 ]
Wang, Fang [1 ]
Wang, Xiaobo [1 ]
Yao, Guihuan [1 ]
机构
[1] Southeast Univ, Minist Educ, Key Lab Energy Thermal Convers & Control, Nanjing 210096, Jiangsu, Peoples R China
关键词
Iron ore; Magnetic field; Magnetically fluidized bed; NO reduction; Selective catalytic reduction; STABILIZED BED; NITRIC-OXIDE; NH3; SCR; NITROGEN; ADSORPTION; AMMONIA; GAS; OXIDATION; MECHANISM;
D O I
10.1002/ceat.201400190
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Low-temperature selective catalytic reduction of NO from simulated flue gas by NH3 on admixtures of iron ore and iron catalyst in a magnetically fluidized bed was experimentally studied. It was found that iron ore exerts a prominent catalytic effect on NO removal resulting in high removal efficiency without magnetic fields. Since iron ore is insensitive to magnetic fields due to its antiferromagnetic property, NO removal efficiency with iron ore as catalyst is only slightly influenced by magnetic fields. The NO removal efficiency, however, can be greatly improved using admixtures of iron ore and iron as catalyst in a magnetically fluidized bed. At defined magnetic field intensity and the same temperature, the removal efficiency reaches higher values compared with that without magnetic fields.
引用
收藏
页码:1537 / 1542
页数:6
相关论文
共 50 条
  • [41] Annealing Strategies for the Improvement of Low-Temperature NH3-Selective Catalytic Reduction Activity of CrMnOx Catalysts
    Zhang, Yanke
    Li, Wan
    France, Liam John
    Chen, Zhihang
    Zeng, Qiang
    Guo, Dawei
    Li, Xuehui
    ACS OMEGA, 2019, 4 (05): : 8681 - 8692
  • [42] Understanding of the high hydrothermal stability of a catalyst prepared from Mn slag for low-temperature selective catalytic reduction of NO
    Hua, Hui
    Zeng, Jiachen
    Wang, Gaorong
    Zhang, Jia
    Zhou, Jizhi
    Pan, Yun
    Liu, Qiang
    Xu, Yunfeng
    Qian, Guangren
    Xu, Zhi Ping
    JOURNAL OF HAZARDOUS MATERIALS, 2020, 381
  • [43] Novel MnOx catalyst for low-temperature selective catalytic reduction of NOx with NH3
    Tang Xiaolong
    Hao Jiming
    Xu Wenguo
    Li Junhua
    CHINESE JOURNAL OF CATALYSIS, 2006, 27 (10) : 843 - 848
  • [44] The influence of chromium substitution on an iron-titanium catalyst used in the selective catalytic reduction of NO
    Karami, Asghar
    Salehi, Vajiheh
    JOURNAL OF CATALYSIS, 2012, 292 : 32 - 43
  • [45] Tungsten modified natural limonite catalyst for efficient low-temperature selective catalytic reduction of NO removal with NH3: preparation and characterization
    Cheng, Ting
    Du, Bo
    Zhou, Huimin
    Jiang, Zhaozhong
    Xie, Qiaoqin
    Zhu, Chengzhu
    ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH, 2023, 30 (13) : 36294 - 36310
  • [46] In situ DRIFTS study of the mechanism of low temperature selective catalytic reduction over manganese-iron oxides
    Chen, Ting
    Guan, Bin
    Lin, He
    Zhu, Lin
    CHINESE JOURNAL OF CATALYSIS, 2014, 35 (03) : 294 - 301
  • [47] The superior performance of CoMnOx catalyst with ball-flowerlike structure for low-temperature selective catalytic reduction of NOx by NH3
    Wang, Zhong-yi
    Guo, Rui-tang
    Shi, Xu
    Liu, Xing-yu
    Qin, Hao
    Liu, Yuan-zhen
    Duan, Chao-peng
    Guo, De-yu
    Pan, Wei-guo
    CHEMICAL ENGINEERING JOURNAL, 2020, 381
  • [48] Improved catalytic activity and N2 selectivity of Fe-Mn-O x catalyst for selective catalytic reduction of NO by NH3 at low temperature
    Xia, Futing
    Song, Zhongxian
    Liu, Xin
    Liu, Xi
    Yang, Yinhua
    Zhang, Qiulin
    Peng, Jinhui
    RESEARCH ON CHEMICAL INTERMEDIATES, 2018, 44 (04) : 2703 - 2717
  • [49] Effects of calcination temperature on Mn species and catalytic activities of Mn/ZSM-5 catalyst for selective catalytic reduction of NO with ammonia
    Lou, Xiaorong
    Liu, Pengfei
    Li, Jun
    Li, Zhe
    He, Kai
    APPLIED SURFACE SCIENCE, 2014, 307 : 382 - 387
  • [50] Low temperature selective catalytic reduction of NO and NO2 with NH3 over activated carbon-supported vanadium oxide catalyst
    Gao, Xiang
    Liu, Shaojun
    Zhang, Yang
    Du, Xuesen
    Luo, Zhongyang
    Cen, Kefa
    CATALYSIS TODAY, 2011, 175 (01) : 164 - 170