Low-Temperature Selective Catalytic Reduction of NO on an Iron Ore Catalyst in a Magnetically Fluidized Bed

被引:16
|
作者
Gui, Keting [1 ]
Liang, Hui [1 ]
Wang, Fang [1 ]
Wang, Xiaobo [1 ]
Yao, Guihuan [1 ]
机构
[1] Southeast Univ, Minist Educ, Key Lab Energy Thermal Convers & Control, Nanjing 210096, Jiangsu, Peoples R China
关键词
Iron ore; Magnetic field; Magnetically fluidized bed; NO reduction; Selective catalytic reduction; STABILIZED BED; NITRIC-OXIDE; NH3; SCR; NITROGEN; ADSORPTION; AMMONIA; GAS; OXIDATION; MECHANISM;
D O I
10.1002/ceat.201400190
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Low-temperature selective catalytic reduction of NO from simulated flue gas by NH3 on admixtures of iron ore and iron catalyst in a magnetically fluidized bed was experimentally studied. It was found that iron ore exerts a prominent catalytic effect on NO removal resulting in high removal efficiency without magnetic fields. Since iron ore is insensitive to magnetic fields due to its antiferromagnetic property, NO removal efficiency with iron ore as catalyst is only slightly influenced by magnetic fields. The NO removal efficiency, however, can be greatly improved using admixtures of iron ore and iron as catalyst in a magnetically fluidized bed. At defined magnetic field intensity and the same temperature, the removal efficiency reaches higher values compared with that without magnetic fields.
引用
收藏
页码:1537 / 1542
页数:6
相关论文
共 50 条
  • [1] Low-Temperature Selective Catalytic Reduction of NO with NH3 over Natural Iron Ore Catalyst
    Husnain, Naveed
    Wang, Enlu
    Fareed, Shagufta
    CATALYSTS, 2019, 9 (11)
  • [2] Magnetic field effects on selective catalytic reduction of NO by NH3 over Fe2O3 catalyst in a magnetically fluidized bed
    Yao, Gui-huan
    Wang, Fang
    Wang, Xiao-bo
    Gui, Ke-ting
    ENERGY, 2010, 35 (05) : 2295 - 2300
  • [3] In situ IR studies of Co and Ce doped Mn/TiO2 catalyst for low-temperature selective catalytic reduction of NO with NH3
    Qiu, Lu
    Pang, Dandan
    Zhang, Changliang
    Meng, Jiaojiao
    Zhu, Rongshu
    Ouyang, Feng
    APPLIED SURFACE SCIENCE, 2015, 357 : 189 - 196
  • [4] Natural manganese ore catalyst for low-temperature selective catalytic reduction of NO with NH3 in coke-oven flue gas
    Zhu, Baozhong
    Yin, Shoulai
    Sun, Yunlan
    Zhu, Zicheng
    Li, Jiaxin
    ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH, 2017, 24 (31) : 24584 - 24592
  • [5] Cerium-loaded MnOx/attapulgite catalyst for the low-temperature NH3-selective catalytic reduction
    Xie, Aijuan
    Zhou, Xingmeng
    Huang, Xiaoyan
    Ji, Liang
    Zhou, Wenting
    Luo, Shiping
    Yao, Chao
    JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY, 2017, 49 : 230 - 241
  • [6] MOF-74 as an Efficient Catalyst for the Low-Temperature Selective Catalytic Reduction of NOx with NH3
    Jiang, Haoxi
    Wang, Qianyun
    Wang, Huiqin
    Chen, Yifei
    Zhang, Minhua
    ACS APPLIED MATERIALS & INTERFACES, 2016, 8 (40) : 26817 - 26826
  • [7] Influence of calcination temperature on iron titanate catalyst for the selective catalytic reduction of NOx with NH3
    Liu, Fudong
    Asakura, Kiyotaka
    He, Hong
    Liu, Yongchun
    Shan, Wenpo
    Shi, Xiaoyan
    Zhang, Changbin
    CATALYSIS TODAY, 2011, 164 (01) : 520 - 527
  • [8] SO2 Deactivation Mechanism of MnOx/MWCNTs Catalyst for Low-Temperature Selective Catalytic Reduction of NOx by Ammonia
    Luo Hong-Cheng
    Huang Bi-Chun
    Fu Ming-Li
    Wu Jun-Liang
    Ye Dai-Qi
    ACTA PHYSICO-CHIMICA SINICA, 2012, 28 (09) : 2175 - 2182
  • [9] Insights into the promotion role of phosphorus doping on carbon as a metal-free catalyst for low-temperature selective catalytic reduction of NO with NH3
    Li, Weifeng
    Jin, Shuangling
    Zhang, Rui
    Wei, Yabin
    Wang, Jiangcan
    Yang, Shuo
    Wang, He
    Yang, Minghe
    Liu, Yan
    Qiao, Wenming
    Ling, Licheng
    Jin, Minglin
    RSC ADVANCES, 2020, 10 (22) : 12908 - 12919
  • [10] BiMnO3 Perovskite Catalyst for Selective Catalytic Reduction of NO with NH3 at Low Temperature
    Zhang Yibo
    Wang Deqiang
    Wang Jing
    Chen Qufei
    Zhang Zhendong
    Pan Xiqiang
    Miao Zhenzhen
    Zhang Bin
    Wu Zhijian
    Yang Xiangguang
    CHINESE JOURNAL OF CATALYSIS, 2012, 33 (09) : 1448 - 1454