Impacts of coal-fired power plants on trace metals and polycyclic aromatic hydrocarbons (PAHs) in lake sediments in central Alberta, Canada

被引:70
作者
Donahue, WF
Allen, EW
Schindler, DW
机构
[1] Univ Alberta, Dept Biol Sci, Edmonton, AB T6G 2E9, Canada
[2] Freshwater Res Ltd, Edmonton, AB T6C 0R6, Canada
基金
加拿大自然科学与工程研究理事会;
关键词
coal combustion; mercury; Pb-210; dating; polycyclic aromatic hydrocarbons; sediment core; trace metals;
D O I
10.1007/s10933-005-7878-8
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Trace metals and polycyclic aromatic hydrocarbons (PAH) were analyzed in sediment cores from three central Alberta lakes to determine the contributions of local coal-red power plants to contaminant loadings. In Wabamun Lake, with four power plants built since 1950 within a 35-km radius, sediment concentrations of mercury, copper, lead, arsenic and selenium have increased by 1.2- to 4-fold. Trace metal enrichments were less pronounced in Lac Ste. Anne and Pigeon Lake, situated 20 km north and 70 km south of Wabamun Lake, respectively. Total Hg flux to Wabamun Lake sediments (21-32 mu g m(-2) yr(-1)) has increased 6-fold since 1950, compared to 2- and 1.5-fold increases in Lac Ste. Anne and Pigeon Lake, respectively, since circa 1900. Total PAH flux to surface sediments was 730-1100 mu g m(-2) yr(-1) in Wabamun Lake, 290-420 mu g m(-2) yr(-1) in Lac Ste. Anne, and 140-240 mu g m(-2) yr(-1) in Pigeon Lake. Without adoption of pollution- abatement technology that compensates for increases in generating capacity, continued expansion of coal-burning industry in Alberta will result in increased contaminant deposition, primarily from local sources.
引用
收藏
页码:111 / 128
页数:18
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